Regional Emissions Analysis of Light-Duty Battery Electric Vehicles

: Light-duty battery electric vehicles (BEVs) can reduce both greenhouse gas (GHG) and criteria air pollutant (CAPs) emissions, when compared to gasoline vehicles. However, research has found that while today’s BEVs typically reduce GHGs, they can increase certain CAPs, though with signiﬁcant regional variability based on the electric grid mix. In addition, the environmental performance of electric and gasoline vehicles is not static, as key factors driving emissions have undergone signiﬁcant changes recently and are expected to continue to evolve. In this study, we perform a cradle-to-grave life cycle analysis using state-level generation mix and vehicle operation emission data. We generated state-level emission factors using a projection from 2020 to 2050 for three light-duty vehicle types. We found that BEVs currently provide GHG beneﬁts in nearly every state, with the median state’s beneﬁt being between approximately 50% to 60% lower than gasoline counterparts. However, gasoline vehicles currently have lower total NOx, urban NOx, total PM 2.5 , and urban PM 2.5 in 33%; 15%; 70%; and 10% of states, respectively. BEV emissions will decrease in 2050 due to a cleaner grid, but the relative beneﬁts when compared to gasoline vehicles do not change signiﬁcantly, as gasoline vehicles are also improving over this time.


Introduction
In 2019, there were 264 million light-duty vehicles (LDVs), with 111 million classified as cars and 153 million as light trucks, in the United States [1]. These vehicles had a significant environmental impact; LDVs accounted for 58% of the greenhouse gas (GHG) emissions from the U.S. transportation sector and for 17% of the U.S. total, in 2019 [2]. Their contributions to criteria air pollutant (CAP) emissions are also significant, as they were responsible for 33% of nitrogen oxide (NOx) emissions and 21% of fine particulate matter (PM 2.5 ) emissions from transportation, which accounted for 20% of total NOx and 4% of PM 2.5 from all anthropogenic sources (excluding fires and dust), in 2017 [3]. Currently, LDV fuel use is dominated by motor gasoline, accounting for 97% of the energy consumed (87% gasoline and 10% ethanol blendstock), while diesel and electricity only account for 2.9% and 0.1%, respectively [1].
Battery electric vehicles (BEVs) have the potential to reduce both GHG and CAP emissions when compared to their gasoline internal combustion engine vehicle (ICEV) counterparts. However, research has found that while today's BEVs typically reduce GHGs, they can increase certain CAPs, though with significant regional variability due to the electrical grid mix [4][5][6][7][8][9].
Cai et al. found BEVs have GHG benefits for national average and select regional grid mixes; in addition, the national average grid mix resulted in higher emissions for NOx and PM 2.5 than a gasoline ICEV, while California and New England grid mixes resulted in lower emissions [4]. Tessum et al. found that a BEV passenger car using grid average electricity increased monetized environmental health impacts (ozone and fine particulates)

Life-Cycle Analysis Modeling Framework
This study used state-of the art modeling from multiple sources to examine the emissions of BEVs and ICEVs using the GREET C2G LCA modeling framework with a system boundary covering both the fuel-cycle and vehicle-cycle. The fuel-cycle examines the environmental impact of production and use of fuels. It includes the following stages: feedstock production; feedstock transportation; fuel production; fuel distribution; and vehicle operation. The fuel-cycle is also called "well-to-wheels", with the stages prior to vehicle operation often called the "upstream" or "well-to-pump" stages, while vehicle operation is also called "pump-to-wheels". The vehicle-cycle examines the production of vehicles. It includes raw material recovery and extraction; material processing and fabrication; vehicle component production; vehicle assembly; and vehicle disposal and recycling. In this study, we used the GREET 2020 model, which included two sub-modules: GREET 1 for fuel-cycle and GREET 2 for vehicle-cycle, to perform our C2G LCA. The GREET model is updated annually with the most up-to-date and detailed energy use and emission data [14]. We used default GREET parameters outside of the changes described in this section. In addition, we used "per vehicle mile driven" as our functional unit, as is standard in GREET.
The GHG emissions we included in this analysis are CO 2 , CH 4 , and N 2 O, which are presented as CO 2e using global warming potentials without climate-carbon feedback from the Intergovernmental Panel on Climate Change's fifth assessment report (AR-5), 1, 30, and 265, respectively [21]. While the GREET model can examine air pollutant emissions, such as carbon monoxide, volatile organic compounds, and PM 10 , in this analysis we focused on NOx and PM 2.5 emissions. We focused on those two CAPs as they have received the most regulatory scrutiny in recent years due to their significant contributions to air quality concerns, such as ozone and fine particulate matter pollution. We further separated the CAP emissions from each source (e.g., coal power plant, oil refineries, and LDVs) into urban and total, to differentiate where they occur and the approximate level of exposure using the GREET model's urban versus rural emission splits [22].

Electricity Grid Mix
We examined the regional and temporal differences of both GHGs and CAPs for BEVs and ICEVs. In general, the GREET model provides U.S. average results; however, it does provide regional data (e.g., generation mixes for each of the North American Electric Reliability Corporation regions). The state-based emission factors presented in this analysis represent the emissions of using BEVs and ICEVs in each state; however, this does not mean we assume all the emission sources for each powertrain reside in every state. For example, some upstream and vehicle-cycle activities occur only in a few states (e.g., vehicle manufacturing), while others may even occur internationally (e.g., crude oil recovery).
In this study, we used state-level generation mixes developed by the National Renewable Energy Laboratory (NREL), published in the Cambium tool [23]. NREL's ReEDS (least-cost utility-scale dispatch) and dGen (distributed solar photovoltaic) models were used to generate 45 forward-looking scenarios of the contiguous U.S. power sector. The scenarios incorporate sensitivities of key factors, such as fuel prices, demand growth, technology costs, and transmission restrictions, resulting in a wide range of possible generation mixes. We selected the reference mid-case 2020 Standard Scenario for the calendar years 2020 to 2050. This scenario uses median assumptions in the models, including existing policies as of June 30, 2020. Figure 1 shows the national average generation mixes for this scenario, with renewable sources growing from 25% in 2020 to 58% in 2050. From this data, we estimated 48 state-level emission factors (excluding Alaska and Hawaii) for each year by applying the state-level generation mixes into the GREET model, as seen in Table A1. generation mixes. We selected the reference mid-case 2020 Standard Scenario for the calendar years 2020 to 2050. This scenario uses median assumptions in the models, including existing policies as of June 30, 2020. Figure 1 shows the national average generation mixes for this scenario, with renewable sources growing from 25% in 2020 to 58% in 2050. From this data, we estimated 48 state-level emission factors (excluding Alaska and Hawaii) for each year by applying the state-level generation mixes into the GREET model, as seen in Table A1.

Vehicle Operation Emission Factors
While GREET uses national average vehicle operation (i.e., "tailpipe") emission factors, we used the recently released MOVES3 model to estimate state-level gasoline ICEV emissions for the model years 2020 to 2050 [24]. We selected three light-duty vehicle types from MOVES to simulate passenger cars, passenger trucks, and light commercial trucks. MOVES emission factors are based on duty-cycle and, therefore, differentiates light commercial trucks, that are primarily used for cargo transport, from passenger trucks, that are primarily used for passenger transport. MOVES defines the duty-cycle based on the fraction of time the vehicle spends in different operating modes (i.e., accelerating, cruise, braking, and idling), with each mode separated by low, medium, and high speeds [25]. MOVES3 LDV NOx emission factors were updated based on millions of results from inuse testing data from the state of Colorado [25]. MOVES3 has lower new LDV NOx emissions and lower NOx deterioration rates as these vehicles age. This results in LDV lifetime weighted NOx emission factors being about half the value they were in the previous version of the model (MOVES2014). However, the LDV PM2.5 emission rates have not changed substantially in the new version.

Vehicle Operation Fuel Consumption
The GREET model uses Argonne's Autonomie vehicle system simulation tool to estimate real-world national average vehicle fuel consumption for select model years, between 2020 and 2050, of various powertrains and vehicle types [26]. Autonomie simulates both low and high technology cases to represent the potential improvement of powertrains in the future; we averaged these cases to represent the fuel consumption for each vehicle and model year combination. Autonomie simulates a midsize passenger car, midsize SUV, and a pickup truck, which we mapped to the MOVES passenger cars, passenger trucks, and light commercial trucks categories, respectively. We selected a BEV with 300 miles of all-electric range on a combined driving cycle (BEV300) to match the current BEV market. As battery technology improves, the typical range may extend past a BEV300. However, a 400 mile BEV's fuel consumption is estimated to be only 5% lower than a BEV300 for MY 2030 and later [26]. In our base case, we assumed the fuel

Vehicle Operation Emission Factors
While GREET uses national average vehicle operation (i.e., "tailpipe") emission factors, we used the recently released MOVES3 model to estimate state-level gasoline ICEV emissions for the model years 2020 to 2050 [24]. We selected three light-duty vehicle types from MOVES to simulate passenger cars, passenger trucks, and light commercial trucks. MOVES emission factors are based on duty-cycle and, therefore, differentiates light commercial trucks, that are primarily used for cargo transport, from passenger trucks, that are primarily used for passenger transport. MOVES defines the duty-cycle based on the fraction of time the vehicle spends in different operating modes (i.e., accelerating, cruise, braking, and idling), with each mode separated by low, medium, and high speeds [25]. MOVES3 LDV NOx emission factors were updated based on millions of results from in-use testing data from the state of Colorado [25]. MOVES3 has lower new LDV NOx emissions and lower NOx deterioration rates as these vehicles age. This results in LDV lifetime weighted NOx emission factors being about half the value they were in the previous version of the model (MOVES2014). However, the LDV PM 2.5 emission rates have not changed substantially in the new version.

Vehicle Operation Fuel Consumption
The GREET model uses Argonne's Autonomie vehicle system simulation tool to estimate real-world national average vehicle fuel consumption for select model years, between 2020 and 2050, of various powertrains and vehicle types [26]. Autonomie simulates both low and high technology cases to represent the potential improvement of powertrains in the future; we averaged these cases to represent the fuel consumption for each vehicle and model year combination. Autonomie simulates a midsize passenger car, midsize SUV, and a pickup truck, which we mapped to the MOVES passenger cars, passenger trucks, and light commercial trucks categories, respectively. We selected a BEV with 300 miles of all-electric range on a combined driving cycle (BEV300) to match the current BEV market. As battery technology improves, the typical range may extend past a BEV300. However, a 400 mile BEV's fuel consumption is estimated to be only 5% lower than a BEV300 for MY 2030 and later [26]. In our base case, we assumed the fuel consumption rates for each powertrain and vehicle combination (e.g., BEV300 passenger truck) was the same in each state. Figure 2 shows the fuel consumption, in gasoline gallon equivalent (GGE) per 100 miles, of BEV300s and gasoline ICEVs from MY 2020 to MY 2050 improving by about 30% and 40%, respectively. In addition, it shows the large discrepancy between the two powertrain types. The absolute difference in fuel consumption difference between each gasoline ICEV type (passenger car vs. passenger truck vs. light commercial truck) is larger than the difference between the BEV300 types. In particular, the gasoline light commercial truck, which is based on a pickup, has much higher fuel consumption than the gasoline passenger vehicles (midsize car and SUV). However, the relative difference between the BEV300 types is larger (light commercial and passenger trucks are 50% and 25% higher than the passenger car) than between the gasoline ICEV types (40% and 10% higher than the passenger car, respectively). The BEV300 fuel (i.e., electricity) consumption on a GGE-basis is between 70% to 75% lower than their gasoline counterparts for all model years. The Autonomie BEV fuel consumption values in Figure 2 are modified when entered into GREET to account for charging losses; we assume a charger efficiency of 85% [27].
consumption rates for each powertrain and vehicle combination (e.g., BEV300 passenger truck) was the same in each state. Figure 2 shows the fuel consumption, in gasoline gallon equivalent (GGE) per 100 miles, of BEV300s and gasoline ICEVs from MY 2020 to MY 2050 improving by about 30% and 40%, respectively. In addition, it shows the large discrepancy between the two powertrain types. The absolute difference in fuel consumption difference between each gasoline ICEV type (passenger car vs. passenger truck vs. light commercial truck) is larger than the difference between the BEV300 types. In particular, the gasoline light commercial truck, which is based on a pickup, has much higher fuel consumption than the gasoline passenger vehicles (midsize car and SUV). However, the relative difference between the BEV300 types is larger (light commercial and passenger trucks are 50% and 25% higher than the passenger car) than between the gasoline ICEV types (40% and 10% higher than the passenger car, respectively). The BEV300 fuel (i.e., electricity) consumption on a GGE-basis is between 70% to 75% lower than their gasoline counterparts for all model years. The Autonomie BEV fuel consumption values in Figure 2 are modified when entered into GREET to account for charging losses; we assume a charger efficiency of 85% [27].

Driving Patterns
Our base case fuel consumption was a composite of city and highway test cycles, weighted 43% and 57%, respectively [28]. This weighting was revised from 55% city and 45% highway to the current values based on a 2006 EPA analysis of fleetwide driver activity data. The study found higher average driving speeds due, in part, to higher speed limits and increased vehicle power over the past two decades since the original values were set [29]. This revision is in contrast to the National Household Travel Survey (NHTS) data that show consistently declining vehicle speeds from 1995 to 2017; however, the NHTS has not historically collected as much data on long-distance travel [30].
Regional driving patterns (i.e., vehicle speed and elevation versus time) will impact the vehicle fuel consumption of different powertrains [7,8]. ICEVs have higher fuel consumption in city driving, which is characterized by low speeds and frequent accelerations, than in highway driving with high speeds and infrequent accelerations [26]. This contrasts with BEVs, which have lower fuel consumption in city driving, due to recaptured energy from regenerative braking [26].
While previous studies have examined the influence of driving patterns, there is a gap in analyzing the impact of vehicle technology advancements. As seen in Figure A1, these improvements impact the fuel consumption difference between driving cycles. The gap between BEV city and highway fuel consumption drops from MY 2020 to MY 2050, due to the improvements in aerodynamics, batteries, electric motors, and lightweighting [26]. The largest improvement is seen for passenger cars, whereby highway driving has

Model Year
Gas light commercial truck Gas passenger truck Gas passenger car BEV300 light commercial truck BEV300 passenger truck BEV300 passenger car

Driving Patterns
Our base case fuel consumption was a composite of city and highway test cycles, weighted 43% and 57%, respectively [28]. This weighting was revised from 55% city and 45% highway to the current values based on a 2006 EPA analysis of fleetwide driver activity data. The study found higher average driving speeds due, in part, to higher speed limits and increased vehicle power over the past two decades since the original values were set [29]. This revision is in contrast to the National Household Travel Survey (NHTS) data that show consistently declining vehicle speeds from 1995 to 2017; however, the NHTS has not historically collected as much data on long-distance travel [30].
Regional driving patterns (i.e., vehicle speed and elevation versus time) will impact the vehicle fuel consumption of different powertrains [7,8]. ICEVs have higher fuel consumption in city driving, which is characterized by low speeds and frequent accelerations, than in highway driving with high speeds and infrequent accelerations [26]. This contrasts with BEVs, which have lower fuel consumption in city driving, due to recaptured energy from regenerative braking [26].
While previous studies have examined the influence of driving patterns, there is a gap in analyzing the impact of vehicle technology advancements. As seen in Figure A1, these improvements impact the fuel consumption difference between driving cycles. The gap between BEV city and highway fuel consumption drops from MY 2020 to MY 2050, due to the improvements in aerodynamics, batteries, electric motors, and lightweighting [26]. The largest improvement is seen for passenger cars, whereby highway driving has about 20% higher fuel consumption than city driving in MY 2020, while it is only 2% higher in MY 2050. For ICEVs, the gap between city and highway fuel consumption widens by about five percentage points from MY 2020 to MY 2050. For our sensitivity case, we examined the impact of state-based driving patterns using MOVES3 vehicle speeds to adjust city and highway weighting based on how each state compares to the national average, as seen in Table A2.

Ambient Temperature
Our base case fuel consumption used adjustment factors to replicate the EPA five-cycle testing method that included both cold and hot temperatures tests. Ambient temperatures impact both vehicle efficiency and loads from heating and air conditioning. Cold temperatures can significantly increase BEV fuel consumption and, thus, EPA five-cycle testing may not be representative of all states [7,8,31]. For our sensitivity case, we applied state-based temperature adjustment factors to the Autonomie fuel consumption values seen in Table A3, based on the piece-wise linear function developed by Wu et al. [8]. Our approach methodology is described in Appendix A.

Vehicle-Cycle Assumptions
The GREET model's vehicle-cycle results were based on a midsize passenger car, midsize SUV, and pickup truck, matching the vehicle types and weights from Autonomie simulations [14,32]. In addition, Argonne's Battery Performance and Cost (BatPaC) model was used to estimate the bill of materials of the lithium-ion nickel manganese cobalt oxide battery chemistry used for the battery LCA in GREET [32,33]. The vehicle-cycle results are provided on a per vehicle basis and are then divided by each vehicle's lifetime mileage (173,151 miles for cars and 183,363 miles for the trucks) to obtain per mile results [32]. We assumed zero battery replacements for the BEVs [34]. In addition, we assumed constant vehicle weight and material composition for each powertrain, and vehicle combination during the analysis period. Thus, vehicle-cycle emissions for each powertrain and vehicle combination do not change from MY 2020 to MY 2050. Figure 3 shows the MY 2020 and MY 2050 national average GHG emission rates for each vehicle type, separated by the fuel-cycle (i.e., upstream and vehicle operation) and vehicle-cycle stages. The error bars show the range of the state-based results. For MY 2020, the vehicle-cycle accounted for approximately 30% of the GHGs for each of the BEV300 vehicle types and 8% for each of the gasoline ICEVs. For MY 2050, it was approximately 50% for BEV300s and 12% for ICEVs. The increase in percentage contribution of the vehicle-cycle for MY 2050 BEV300s was due to the reduction in upstream emission from the increased amount of renewable electricity generation, as seen in Figure 1, and also an increase in vehicle fuel efficiency, as seen in Figure 2.  Figure 4 shows the state-based C2G (fuel-cycle and vehicle-cycle) GHG emission rates of BEV300 passenger trucks for MY 2020 and MY 2050 for both the base and sensitivity cases. While the state-based emission benefits in Figure 4 are not the same for passenger cars and light commercial trucks (see Figures C1 and C2), the relative difference (i.e. map shading) is similar. For MY 2020, upstream sources accounted for about 70% of GHGs for each BEV300 vehicle type and 17% for the gasoline ICEVs. For MY 2050, it was approximately 50% for BEV300s and, again, 17% for ICEVs. BEVs did not have any vehicle operation GHGs, while the gasoline ICEV GHGs were dominated by this source: 75% for MY 2020 and 70% for MY 2050. In this study, the change in grid mix accounted for a significant portion (~75%) of the improvement in BEV300 GHG emission rates from MY 2020 to MY 2050, with the rest being due to fuel efficiency. Fuel efficiency improvements accounted for the entire reduction in gasoline ICEV GHGs over the study period. Figure 4 shows the state-based C2G (fuel-cycle and vehicle-cycle) GHG emission rates of BEV300 passenger trucks for MY 2020 and MY 2050 for both the base and sensitivity cases. While the state-based emission benefits in Figure 4 are not the same for passenger cars and light commercial trucks (see Figures A2 and A3), the relative difference (i.e. map shading) is similar.  Figure 4 shows the state-based C2G (fuel-cycle and vehicle-cycle) GHG emission rates of BEV300 passenger trucks for MY 2020 and MY 2050 for both the base and sensitivity cases. While the state-based emission benefits in Figure 4 are not the same for passenger cars and light commercial trucks (see Figures C1 and C2), the relative difference (i.e. map shading) is similar.  For MY 2020, the only states in which BEV300 passenger truck GHG emission rates were higher than the gasoline ICEV counterpart were Kentucky, in both cases, and Wyoming, joining it in the sensitivity case. For MY 2020, six other states (Indiana, Missouri, West Virginia, Utah, Ohio, and Wisconsin) had BEV300 emission rates resulting in less than 25% GHG reduction versus gasoline ICEV passenger trucks. Conversely, in 2020  For MY 2020, the only states in which BEV300 passenger truck GHG emission rates were higher than the gasoline ICEV counterpart were Kentucky, in both cases, and Wyoming, joining it in the sensitivity case. For MY 2020, six other states (Indiana, Missouri, West Virginia, Utah, Ohio, and Wisconsin) had BEV300 emission rates resulting in less than 25% GHG reduction versus gasoline ICEV passenger trucks. Conversely, in 2020 Vermont generated 100% of its electricity from renewable sources, so the state's only BEV300 GHG emissions were from the vehicle-cycle. For MY 2020, three other states (New Hampshire, Montana, and Washington) had BEV300 emission rates resulting in more than 80% reduction versus gasoline ICEV passenger trucks.

GHG Emissions
The state-based city and highway driving percentages (see Table A2) resulted in a maximum BEV300 fuel consumption increase of 3% for South Dakota (highest highway percentage) and decrease of 1.5% for Florida (highest city percentage) MY 2020 light commercial trucks. For ICEVs, the pattern was reversed with a 3% decrease for South Dakota and increase of 1.5% for Florida for MY 2050 passenger cars. Factors, such as aerodynamic drag, impacted these changes, with the more aerodynamic MY 2020 BEV types having a smaller fuel consumption increase in South Dakota (approximately 2% for passenger cars and 2.5% for passenger trucks) than the light commercial truck value of 3%.
The state temperature adjustment factors (see Table A3) resulted in an increase in fuel consumption of approximately 15% for BEVs and 4% for ICEVs, on average. For cold weather states like North Dakota, Minnesota, and Wyoming, the adjustment factors can result in an increase in fuel consumption of approximately 25% for BEVs and 7% for ICEVs. For warm weather states like Florida, Louisiana, and Georgia they result in an increase of less than 5% for BEVs and 2% for ICEVs.
As seen in Figure A4, the two fuel consumption adjustments result in the median state's BEV300 passenger truck having less GHG benefits versus the ICEV, 5 g/mi in MY 2020 and 9 g/mi in MY 2050, when compared to the base case. In MY 2020, the sensitivity case had a broader range of impacts with the BEV300 having 78 g/mi less benefits in Wyoming due to cold weather and high-speed driving. Conversely, the sensitivity case was 19 g/mi better in New Hampshire and Vermont for the BEV300. This was due to the clean grid mix not being impacted by increased vehicle fuel consumption from the cold weather (e.g., 20% higher fuel consumption for a zero emission vehicle is still zero). The range of impacts flattened for MY 2050 due to the relative improvement of BEV300 highway fuel consumption.
As seen in Figures 4 and 5, BEV300s provide significant GHG benefits versus their gasoline ICEV counterparts in nearly every state. For the MY 2020 base case, the median state had 57%, 52%, and 54% lower GHG emission rates for a BEV300 than its gasoline passenger car, passenger truck, and light commercial truck counterpart, respectively. While Figure 4 shows that the absolute g/mi benefits decrease for MY 2050, Figure 5 shows the relative benefits increase slightly. For the MY 2050 base case, the median state's BEV300s had 64%, 60%, and 61% lower GHG emission rates, respectively. For the sensitivity case, relative benefits of BEV300s on average decreased less than five percentage points for both model years. For MY 2020, upstream sources accounted for about 60% of the total NOx and 80% of urban NOx for each BEV300 vehicle type; for MY 2050 the upstream contributions were lower as the grid increasingly used renewables, 30% and 60%, respectively. BEVs did not have any vehicle operation NOx. Gasoline ICEV NOx vehicle operation accounted for approximately only 20% of total NOx and 50% of urban NOx for both model years. In addition, Figure 5 shows that for each model year and vehicle type combination, three-quarter of the states (third quartile) have at least 35% reduction in GHGs, while one-quarter (first quartile) have more than 60% reduction. The maximum GHG percentage reduction for BEV300s decreased for MY 2050 due to the improvements in gasoline fuel consumption rates, even though Virginia, in 2050 has an upstream GHG emission rate of less than 0.3 g/mi, due to its 76% renewables and 24% nuclear generation mix. Figure 6 shows the MY 2020 and MY 2050 national average total and urban NOx emission rates for each vehicle type, with the error bars showing the range of the statebased results. For MY 2020, the vehicle-cycle accounted for about 40% of the total NOx and 20% of urban NOx for each BEV300 vehicle type. For MY 2050 BEVs, it was 70% and 40%, respectively. For gasoline ICEVs, the vehicle-cycle contribution was about half that of the BEV percentages.  Figure 6 shows the MY 2020 and MY 2050 national average total and urban NOx emission rates for each vehicle type, with the error bars showing the range of the statebased results. For MY 2020, the vehicle-cycle accounted for about 40% of the total NOx and 20% of urban NOx for each BEV300 vehicle type. For MY 2050 BEVs, it was 70% and 40%, respectively. For gasoline ICEVs, the vehicle-cycle contribution was about half that of the BEV percentages.

Total and Urban NOx
For MY 2020, upstream sources accounted for about 60% of the total NOx and 80% of urban NOx for each BEV300 vehicle type; for MY 2050 the upstream contributions were lower as the grid increasingly used renewables, 30% and 60%, respectively. BEVs did not have any vehicle operation NOx. Gasoline ICEV NOx vehicle operation accounted for approximately only 20% of total NOx and 50% of urban NOx for both model years. As seen in Figures 6 and 7, BEV300s can provide NOx benefits in some states. However, Figure 7   For MY 2020, upstream sources accounted for about 60% of the total NOx and 80% of urban NOx for each BEV300 vehicle type; for MY 2050 the upstream contributions were lower as the grid increasingly used renewables, 30% and 60%, respectively. BEVs did not have any vehicle operation NOx. Gasoline ICEV NOx vehicle operation accounted for approximately only 20% of total NOx and 50% of urban NOx for both model years.
As seen in Figures 6 and 7, BEV300s can provide NOx benefits in some states. However, Figure 7 shows the near universal state-based GHG benefits of BEV300s does not apply to NOx emissions. For MY 2020, approximately 33% of states had lower total NOx emissions for the gasoline ICEVs; for MY 2050, it was 20% of the states. For MY 2020, approximately 15% of states had lower urban NOx emissions for the gasoline ICEVs; for MY 2050, it was only 5% of states. Figure 7 shows that for MY 2020, the median state in the base case has 15%, 9%, and 9% lower total NOx emission rates for a BEV300 than its gasoline passenger car, passenger truck, and light commercial truck counterpart, respectively. For MY 2050, the median state's benefit in the base case increased slightly with BEV300s having 24%, 19%, and 19% lower total NOx emission rates, respectively.
BEV300s provided more urban than total NOx benefits. For MY 2020, the median state in the base case had 58%, 56%, and 55% lower urban NOx emission rates for a BEV300 than its gasoline counterpart, respectively. For MY 2050, the median state's benefit in the base case also increased slightly with BEV300s having 66%, 64%, and 65% lower urban NOx emission rates, respectively. For the sensitivity case, the relative benefits of BEV300s, on average, decreased approximately five percentage points for both total and urban NOx in both model years.
state in the base case had 58%, 56%, and 55% lower urban NOx emission rates for a BEV300 than its gasoline counterpart, respectively. For MY 2050, the median state's benefit in the base case also increased slightly with BEV300s having 66%, 64%, and 65% lower urban NOx emission rates, respectively. For the sensitivity case, the relative benefits of BEV300s, on average, decreased approximately five percentage points for both total and urban NOx in both model years.  Figure 8 shows the MY 2020 and MY 2050 national average total and urban PM2.5 emission rates for each vehicle type, with the error bars showing the range of the statebased results. For MY 2020, the vehicle-cycle accounted for about 50% of the total PM2.5 and only 5% of urban PM2.5 for each BEV300 vehicle type. For MY 2050 BEV300s, it was 60% and 10%, respectively. For MY 2020 gasoline ICEVs, the vehicle-cycle accounted for about 30% of the total PM2.5 and only 5% of urban PM2.5. For MY 2050 ICEVs, it was 35% and 5%, respectively.
For MY 2020, upstream sources accounted for about 35% of both the total PM2.5 and urban PM2.5 for each BEV300 vehicle type. For MY 2050 BEV300s, the upstream   As seen in Figures 8 and 9, BEV300s can provide PM2.5 benefits in some states. However, the case is similar to NOx, where in many states BEVs do not have lower PM2.5 emissions. This is especially the situation for total PM2. 5   For MY 2020, upstream sources accounted for about 35% of both the total PM 2.5 and urban PM 2.5 for each BEV300 vehicle type. For MY 2050 BEV300s, the upstream contributions were lower as the grid increasingly used renewables, 15% and 20%, respectively. Unlike NOx (and all other CAP emissions), BEVs do produce vehicle operation PM 2.5 from tire and brake wear (TBW). For MY 2020 BEV300s, TBW accounted for approximately 20% of total PM 2.5 and 60% of urban PM 2.5 . For MY 2050 BEV300s, it was 25% and 75%, respectively. For MY 2020 gasoline ICEVs, PM 2.5 vehicle operation (tailpipe and TBW) accounted for about 33% of total PM 2.5 and 60% of urban PM 2.5 . For MY 2050 ICEVs, it was nearly 40% and 70%, respectively.
As seen in Figures 8 and 9, BEV300s can provide PM 2.5 benefits in some states. However, the case is similar to NOx, where in many states BEVs do not have lower PM 2.5 emissions. This is especially the situation for total PM 2.5 emissions. For MY 2020, about 70% of states had lower total PM 2.5 emissions for the gasoline ICEVs; for MY 2050, it was 60% of the states. For MY 2020, about 10% of states had lower urban PM 2.5 emissions for the gasoline ICEVs, but none of states were lower for MY 2050.

Discussion and Conclusions
The ability of light-duty BEVs to provide GHG and CAP benefits is strongly dependent on the grid mix powering the vehicle, BEV efficiency, and the relative performance of gasoline ICEV counterparts. Due to the regional differences in electricity generation, the potential benefits are not evenly distributed across all U.S. states. In addition, as grid is decarbonizing, the magnitude of potential benefits is changing quickly.
Our analysis demonstrates that BEV300s currently provide GHG benefits in nearly every state, with the median state's BEV300 emission rate being between 50% to 60% lower than their gasoline ICEV passenger car, passenger truck, and light commercial truck counterparts. As the grid incorporates more renewables in our scenario, from 2020 to 2050, absolute BEV300 GHG emission rates decrease by 40%, but due to the improvements for ICEVs the relative benefits do not change significantly. How the grid will evolve over the next 30 years is difficult to predict, as can be seen by the in NREL's Standard Scenarios  Figure 9 shows that for MY 2020, the median state in the base case has 9%, 12%, and 12% higher total PM 2.5 emission rates for a BEV300 than its gasoline passenger car, passenger truck, and light commercial truck counterpart, respectively. For MY 2050, the median state's BEV300s in the base case had the same, 3% higher, and 4% higher total PM 2.5 emission rates, respectively.
BEV300s provided more urban than total PM 2.5 benefits. For MY 2020, the median state in the base case had 34%, 34%, and 35% lower urban PM 2.5 emission rates for a BEV300 than its gasoline counterpart, respectively. For MY 2050, the median state's benefit in the base case also increased slightly with BEV300s having 41%, 39%, and 41% lower urban PM 2.5 emission rates, respectively. For the sensitivity case, relative benefits of BEV300s on average decreased by about five percentage points for both total and urban PM 2.5 in both model years.

Discussion and Conclusions
The ability of light-duty BEVs to provide GHG and CAP benefits is strongly dependent on the grid mix powering the vehicle, BEV efficiency, and the relative performance of gasoline ICEV counterparts. Due to the regional differences in electricity generation, the potential benefits are not evenly distributed across all U.S. states. In addition, as grid is decarbonizing, the magnitude of potential benefits is changing quickly.
Our analysis demonstrates that BEV300s currently provide GHG benefits in nearly every state, with the median state's BEV300 emission rate being between 50% to 60% lower than their gasoline ICEV passenger car, passenger truck, and light commercial truck counterparts. As the grid incorporates more renewables in our scenario, from 2020 to 2050, absolute BEV300 GHG emission rates decrease by 40%, but due to the improvements for ICEVs the relative benefits do not change significantly. How the grid will evolve over the next 30 years is difficult to predict, as can be seen by the in NREL's Standard Scenarios report outputting a wide range of potential future generation mixes [23]. However, if the U.S. is able to meet goals, such as decarbonizing the grid by 2035, the benefits of BEVs will be larger and faster than the mid-case scenario we analyzed [35].
Vehicle-cycle activities becomes a larger proportion of GHGs as the grid becomes cleaner. Further analysis should be done to examine how the vehicle-cycle emissions will change into the future. For example, the vehicle production can involve heavy industrial activities (e.g., iron smelting and steelmaking), which will be difficult, but not impossible, to decarbonize [36]. However, some vehicle-cycle activities (e.g., aluminum refining and several vehicle assembly stages), can be electricity intensive, so changes in the grid will not only impact BEV upstream emissions but also the vehicle-cycle.
In our sensitivity case, we examined the impacts of driving patterns and ambient temperature on state-based fuel consumption rates of BEVs and ICEVs. BEVs have greater fuel efficiency benefits over ICEVs in stop-and-go duty-cycles due to factors, such as regenerate braking, when compared to highway driving. Furthermore, we found that states that have a significant amount of highway driving can increase BEV fuel consumption by up to 3% versus our base case, while reducing fuel consumption by 1.5% in states with significant city driving. In contrast, ICEV fuel consumption can decrease by up to 3% in states with a lot of highway driving and decrease by 1.5% with a lot of city driving. Ambient temperatures can have an even greater impact on fuel consumption, especially for BEVs. For cold weather states, BEV and ICEV fuel consumption can increase by up to 25% and 7%, respectively, while for warm weather states, it can increase by up to 5% for BEVs and 2% for ICEVs.
For CAP emissions, differences in emission source location and rates are key factors to understand the potential of BEVs to provide air quality benefits. Our analysis demonstrates that the near universal state-based GHG benefits of BEV300s does not apply to NOx and PM 2.5 emissions. Currently, gasoline ICEVs have lower total NOx and total PM 2.5 in 33% and 70% of states, respectively; while in 2050, these number will drop to 15% and 60% in our scenario.
However, our study found that BEV300s can provide significant urban NOx and urban PM 2.5 benefits. Currently, the median state's urban NOx benefit for BEV300s is approximately 60% lower than gasoline ICEVs for the three vehicle types we studied; for urban PM 2.5 the median state's benefit is approximately 35%. Again, we see the benefit increasingly slightly as the grid decarbonizes in the future though the benefits are mitigated due to gasoline ICEV improvements.
The results of our study can be used in conjunction with state-based adoption modeling to understand implications of the regional variation in both emission rates and activity to estimate annual emission changes. Regional activity will depend on both the LDV population and annual vehicle miles traveled in each state. The potential BEV emission benefits depend not only on relative emission rates calculated in this study, but the number of BEVs being purchased. Therefore, particular attention should be paid to states with large vehicle populations. With that data, the emission rates from our LCA study can be used with air quality modeling (e.g., chemical transport models and reduced complexity models) to better understand the health impacts of BEVs. Using the latest modeling and data, regional LCA can be helpful in addressing both global issues, like GHG emissions, and local issues local, like the environmental justice impacts, from the adoption of BEVs. The views and opinions of the authors expressed herein do not necessarily state or reflect those of the U.S. Government or any agency thereof. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights.

Institutional Review Board Statement: Not applicable.
Informed Consent Statement: Not applicable.

Data Availability Statement:
All the data supporting the findings of this study are included in this article.

Conflicts of Interest:
The authors declare no conflict of interest.      where r T is the fuel consumption ratio (relative to operation in the efficiency plateau of 15.5-23.9 • C) at temperature T. The values of coefficient a 1 are 0.0129 and 0.0210 for the ICEV and BEV, respectively. The values of coefficient a 2 are 0.0064 and 0.0242 for ICEV and BEV, respectively. Table A3 shows the annual-average state temperature adjustment factors for vehicle fuel consumption for ICEVs and BEVs. The state temperatures for the calendar year 2020 are based on the National Oceanic and Atmospheric Administration (NOAA) dataset [38].    (a) (b) Figure A3. Change in GHG emission rate of BEV300 versus ICEV light commercial trucks by state for 2020 and 2050. Blue indicates states BEV300s have lower emissions than ICEVs, while red indicates BEV300s have higher emissions than ICEVs.

Appendix A. State Generation Mixes
(a) Base case with no fuel consumption adjustments, and (b) sensitivity case with fuel consumption adjustments. Figure A4. Change in GHG emission rate of BEV300 versus ICEV passenger trucks in sensitivity case versus base case. The negative values indicate that states in sensitivity case have larger BEV300 GHG benefits versus ICEV than they do in base case. The positive values indicate that states in sensitivity case have lower BEV300 GHG benefits versus ICEV than they do in base case. Figure A4. Change in GHG emission rate of BEV300 versus ICEV passenger trucks in sensitivity case versus base case. The negative values indicate that states in sensitivity case have larger BEV300 GHG benefits versus ICEV than they do in base case. The positive values indicate that states in sensitivity case have lower BEV300 GHG benefits versus ICEV than they do in base case.