Investigation of the Impact of Micro-Structuring on the Bonding Performance of Beechwood (Fagus Sylvatica L.)

Although glueing softwood is well mastered by the industry, predicting and controlling bond quality for hardwood is still challenging after years of research. Parameters such as the adhesive type, resin–hardener ratio, and the penetration behaviour of the wood are determinants for the bond quality. The aim of this work was to assess to what extent the glueing behaviour of beechwood can be improved by using structural planing. The different surfacing methods were characterised by their roughness. The bond strength of the micro-structured surfaces was determined according to EN 302-1, and the delamination resistance was tested as indicated by EN 302-2 for type I adhesives. Microstructured surfaces were compared with different surfaces (generated by surfacing methods such as dull/sharp planing and sanding). In dry test conditions, all surfacing methods gave satisfying results. In the wet stage, the bond strength on the finer micro-structured surface slightly outperformed the coarse structure surface. For the delamination resistance, a clear improvement could be observed for melamine-formaldehyde-bonded specimens since, when using the recommended amount of adhesive, micro-structured surfaces fulfilled the requirements. Nevertheless, structural planing cannot lead to a reduction in the applied grammage since no sample with a smaller amount fulfilled EN 302-2 requirements even by observing the recommended closed assembly waiting time. Adhesion area enlargement of the micro-structuring is minor. The good delamination performance without waiting time (CAT) is not caused by surface enlargement, since finer micro-structured surface with negligible area increase and delivered even better delamination resistance. Subsurface analysis should be carried out to thoroughly investigate this phenomenon.


Introduction
In Switzerland, softwoods account for most of the wood processed each year for various construction applications. Moreover, beechwood has a yearly growth of around 2 million cubic metres, whereas spruce has 5 million cubic metres. There is a clear dominance of softwoods in the construction market. In Switzerland, each time that a million cubic metres of spruce are used, only 36,000 cubic metres of beechwood are used [1]. This notable difference is mainly explained by the orientation of the wood industry.
Furthermore, the fact that spruce is a limited resource motivates research into the development of processing techniques for the optimal use of hardwoods. The superior mechanical properties of beech and the large reserves present in Switzerland make it the ideal candidate to try to rebalance the construction market. Due to the low utilisation of hardwoods in Central Europe, hardwood-processing techniques have not yet reached a similar technological development level as softwoods. the chosen pattern. It is commonly accepted that rougher surfaces provide better adhesion smoother surfaces.
To achieve successful glueing of hardwood, the use of long-closed assembly time is required when using melamine urea-formaldehyde (MUF) or melamine-formaldehyde (MF) systems. This waiting time can even be longer than an hour when working with MUF [2,28]. When using one-component polyurethane adhesive, it was not possible to pass the delamination test according to EN 302-2 without using surface chemical pretreatment [12].
Micro-structuring has its roots in the field of surface coating. It has been shown that through structured planing of the surface to coat, the coating durability was increased [29]. Investigations have been made on softwoods used for outdoor applications, where better durability of the adhesion between the wood and coating is required. The durability of the adhesion refers to its resistance against adverse climate conditions (humidity, insolation).
Lehmann and Volkmer [3] investigated the bond quality of micro-structured surfaces for hardwoods. They used three different wood species: ash (Fraxinus excelsior L.), beech (Fagus Sylvatica L.), and spruce (Picea abies Karst.). The microstructure machined on the surface was observed by optical microscopy. The profile depth was reported to be 43 µm, as can be observed in Figure 1. They conducted investigations of glue lines carried out with PUR (without primer) and MUF. Those series underwent a delamination test in respect to EN 302-2. The results showed that for MUF, the one-sided micro-structure planing of specimens had a promising impact on bond quality. They reported that no closed assembly time was needed to meet the delamination requirement for MUF. On the other hand, although the influence of micro structuring was still visible on samples adhesively joined with PUR, the delamination values were far above the accepted threshold. The PUR without primer performed poorly when used on hardwood. It was also observed that onesided micro-structuring delivers better results than double-sided micro-structuring. PUR samples could fulfil neither the low nor the high-temperature process of EN 302-2 standard. The glulam layup of that experiment made micro-structured and normally planed surfaces within the same board. This might also have influenced the results since once the weakest bond line fails, the other bond lines are destressed and experience less delamination. The form factor can also be considered since it is known that a smaller sample dimensions for delamination with hardwood can improve the test results [30]. To achieve successful glueing of hardwood, the use of long-closed assembly time is required when using melamine urea-formaldehyde (MUF) or melamine-formaldehyde (MF) systems. This waiting time can even be longer than an hour when working with MUF [2,28]. When using one-component polyurethane adhesive, it was not possible to pass the delamination test according to EN 302-2 without using surface chemical pretreatment [12].
Micro-structuring has its roots in the field of surface coating. It has been shown that through structured planing of the surface to coat, the coating durability was increased [29]. Investigations have been made on softwoods used for outdoor applications, where better durability of the adhesion between the wood and coating is required. The durability of the adhesion refers to its resistance against adverse climate conditions (humidity, insolation).
Lehmann and Volkmer [3] investigated the bond quality of micro-structured surfaces for hardwoods. They used three different wood species: ash (Fraxinus excelsior L.), beech (Fagus Sylvatica L.), and spruce (Picea abies Karst.). The microstructure machined on the surface was observed by optical microscopy. The profile depth was reported to be 43 μm, as can be observed in Figure 1. They conducted investigations of glue lines carried out with PUR (without primer) and MUF. Those series underwent a delamination test in respect to EN 302-2. The results showed that for MUF, the one-sided micro-structure planing of specimens had a promising impact on bond quality. They reported that no closed assembly time was needed to meet the delamination requirement for MUF. On the other hand, although the influence of micro structuring was still visible on samples adhesively joined with PUR, the delamination values were far above the accepted threshold. The PUR without primer performed poorly when used on hardwood. It was also observed that onesided micro-structuring delivers better results than double-sided micro-structuring. PUR samples could fulfil neither the low nor the high-temperature process of EN 302-2 standard. The glulam layup of that experiment made micro-structured and normally planed surfaces within the same board. This might also have influenced the results since once the weakest bond line fails, the other bond lines are destressed and experience less delamination. The form factor can also be considered since it is known that a smaller sample dimensions for delamination with hardwood can improve the test results [30]. The aim of this study was to assess the impact of surface preparation on the bondability of beechwood. The characterisation of the micro-structured surfaces and the use of  The aim of this study was to assess the impact of surface preparation on the bondability of beechwood. The characterisation of the micro-structured surfaces and the use of different adhesives with various process parameters aimed to gather knowledge about the extent of the positive effects of structural planing can already be observed in previous studies [3]. For this study, it was assumed that structural planing improves the mechanical performance of a bond line, and therefore less-demanding requirements on the adhesive to be employed were expected.

Bonding Parameters and Test Specimens
All adhesive-based connections carried out have involved beechwood (Fagus sylvatica L.). For the tensile shear test, the growth ring angle (GRA) ranges from 60 to 85 to lessen the wood impact. It is known that flat growth ring angle is associated with poor bonding performance [27,32]. The beech boards were conditioned in normal climate (20 • C/65% relative humidity) until the equilibrium moisture content of 12% was reached (14 days). In these conditions, the average density ρ of the boards was (700 ± 50) kg/m 3 . Five different surface preparations were compared (sharp planing, planing with dull knives, sanding, and structural planing with coarse and fine patterns). Sharp planing was realised with a set of new and unused knives, whereas the dull knives, engaged for the creation of dull planed surfaces, were chosen among knives at the end of tool life. To obtain micro-structured surfaces, knives with pre-defined profiles in the back of the blade were used. Both used structures represented in Figure 2a,b. They, respectively, represent the coarse and fine structures. To assess the impact of surface preparation on bonding performance, a tensile shear test was carried out according to EN 302-1 [33]. The different surfaces produced are summed up in Table 1. different adhesives with various process parameters aimed to gather knowledge about the extent of the positive effects of structural planing can already be observed in previous studies [3]. For this study, it was assumed that structural planing improves the mechanical performance of a bond line, and therefore less-demanding requirements on the adhesive to be employed were expected.

Bonding Parameters and Test Specimens
All adhesive-based connections carried out have involved beechwood (Fagus sylvatica L.). For the tensile shear test, the growth ring angle (GRA) ranges from 60 to 85 to lessen the wood impact. It is known that flat growth ring angle is associated with poor bonding performance [27,32]. The beech boards were conditioned in normal climate (20 °C /65% relative humidity) until the equilibrium moisture content of 12% was reached (14 days). In these conditions, the average density of the boards was (700 ± 50) kg/m 3 . Five different surface preparations were compared (sharp planing, planing with dull knives, sanding, and structural planing with coarse and fine patterns). Sharp planing was realised with a set of new and unused knives, whereas the dull knives, engaged for the creation of dull planed surfaces, were chosen among knives at the end of tool life. To obtain microstructured surfaces, knives with pre-defined profiles in the back of the blade were used. Both used structures represented in Figure 2a,b. They, respectively, represent the coarse and fine structures. To assess the impact of surface preparation on bonding performance, a tensile shear test was carried out according to EN 302-1 [33]. The different surfaces produced are summed up in Table 1.    The adhesive was applied one-sidedly with a grammage set to 125 g m 2 with a wooden spatula. A lower grammage was used to cause failure at the interface. This a one-component polyurethane with a 30-min assembly time is used for structural applications with softwood and is available under the commercial name HBS 309 (PUREBOND ® , Sempach, Switzerland). A one-component PUR adhesive was purposely chosen to achieve adhesive failure and remove the influence of the wood choice on the result since the wood failure percentage is lessened to its minimum.
The micro-structured prefabricated boards deviate from the standards (EN 205 [34]) since the folding could not be respected to guarantee to have one-sided micro-structured joints. It is known that one-sided structuring performs better [3]. The board was turned to obtain a fishbone pattern. Another difference to the standards is caused by the minimum thickness to be set on the four-face-planer, which is 9.5 mm. Going under this value causes a collision between the upper cutter head and the inner table, with severe damages to the machine. Therefore, the micro-structured prefabricated boards were 20 mm thick and had to be planed down to 10 mm on a regular thickness planer (with an equal removal of 5 mm on each side). Glueing parameters, such as open/closed assembly time (OAT/CAT), are listed in Table 2. Roughness measurement occurred within 24 h after machining. The surface roughness parameter R a (arithmetic mean of the absolute ordinate values) was determined on a measuring length of 4 mm with a cutoff length of 0.5 mm at a measuring speed of 0.5 mm s −1 . The measurement was realised using the Surftest SJ 210 roughness tester (© Mitutoyo, Urdorf, Switzerland, which uses the stylus method) in accordance with EN ISO 4287:2010 [35]. The roughness was measured in the cross-grain direction.

Test Set-Up and Bonding Parameters
In order to assess the impact of micro-structuring (S1 and S2 as defined in Table 1), six groups of samples were defined for each adhesive involved (1C PUR and MF). For the micro-structured (S1 and S2) and normally planed surfaces, two different grammages were tested. The normally planed surface was used as a benchmark. The polyurethane adhesive used for this part of the experiments is commercially available under the name: HB S109 (PUREBOND ® , Sempach, Switzerland). The melamine-formaldehyde system used is a formulation from AkzoNobel commercialised as GripPro TM Design (Akzo Nobel, Kristinehamn, Sweden). The process parameters are reported in Table 3. Table 3. Glueing parameters and adhesive information at 20 • C. Adhesive was applied on sample in the laboratory at 20 • C and 65% relative humidity. Melamine formaldehyde was mixed with a resin-hardener mixing ratio of 100:50 (by weight). Different grammages were considered to assess the impact of micro-structuring (S1 and S2) on bond quality.

Tensile Shear Test
For the assessment of the adhesive performance, shear tests in both dry and wet stages were carried out. A1 and A4 treatments were undertaken.
Wood. All the prefabricated boards were made from beechwood (Fagus sylvatica L.). The wood was selected according to SN EN 302-1:2013. The wood used for the test were rift sawn with GRA ranging from 60 • to 85 • . The beech boards were conditioned in normal climate (20 • C/65% relative humidity) until the equilibrium moisture content of 12% was reached. In these conditions, the measured average density ρ of the boards was (700 ± 50) kg/m 3 .
Test Procedure. After the glueing, the boards were stored in normal climate for at least a week. After, the test specimens were produced according to EN 205. The density of each specimen was determined before executing the tensile shear test. The specimens were tested at a constant testing speed, in force-controlled mode (2 kN/min) as indicated by the standards.
Evaluation method. The evaluation was based on the EN 302-1(2013). Data were censored in cases where the groove was not properly executed. As a deviation from the standards, the selection of a pre-defined sample size was carried out through randomisation. This randomisation occured in matlab with an algorithm that selects distinct sample from the censored raw data randomly (to avoid duplicates). This deviation from the norm makes sense since the aim of this research work is not to analyse an adhesive but to compare different surface treatments. The sample size used for the comparison of the different series was set to ten. Randomisation was not applied to the samples tested in dry stage since the initial sample size was set to 10. For the wet-stage tensile-shear-strength test, 30 samples per group were produced and tested, but only the limited sample size of 10 was evaluated after randomisation.

Delamination Test
To compare the bond performance of the structural planing, delamination tests were carried out on beechwood (Fagus Sylvatica L.). The selected wood had flat growth ring angle as recommended by the standard EN 302-2. The wood was first climatised in normal climate (20 • C/65% relative humidity) until the equilibrium moisture content of 12% was reached. The measured average density ρ of the boards was (687 ± 27) kg/m 3 . Wood was sorted in respect to density, and density classes were defined as follows: C1 (627-662 kg/m 3 ); C2 (662-697 kg/m 3 ); C3 (697-732 kg/m 3 ).
The first two lamellae are from class C1, the middle pair of lamellae are from the C3 class, and the last pair is from the C2 class. This layup was respected for all delamination samples. Due to production capacity, the length of the glulam was limited to 250 mm, and one delamination sample was extracted out of the glulam.
Delamination tests were carried out on two different adhesive systems. Since both adhesive systems used are certified for structural applications, the high-temperature procedure suited to type I adhesives was applied. However, the one-component polyurethane (1C PUR) did not undergo a surface reactivation through the usage of primer solution, which exposes it to bad delamination performance on hardwood [36]. The process parameters are represented in Table 4.  Figure 3 shows a comparison of all the machining methods used in this work. The coarse structure has the highest Ra value, followed by the fine structure, which has a lower roughness in comparison. The normally planed surface has a lower roughness than the poorly planed and sanded surfaces. The poorly planed surface had a lower dispersion and was even smoother than sanding with a P100 grit. Statistic investigations by means of Kruskal-Wallis and Dunn's post hoc test revealed no significant differences between the roughness obtained for sanding and dull planing (p = 0.7 > 0.05) at the significance level of 5%. Normally planed (with sharp knives) and coarsely micro-structured produce surfaces significantly different in terms of roughness (p = 1.06 × 10 −7 < 0.05). The fine micro-structuring also showed a significant difference compared to the normal planing (p = 1.37 × 10 −2 < 0.05).  Figure 3 shows a comparison of all the machining methods used in this work. The coarse structure has the highest Ra value, followed by the fine structure, which has a lower roughness in comparison. The normally planed surface has a lower roughness than the poorly planed and sanded surfaces. The poorly planed surface had a lower dispersion and was even smoother than sanding with a P100 grit. Statistic investigations by means of Kruskal-Wallis and Dunn's post hoc test revealed no significant differences between the roughness obtained for sanding and dull planing ( = 0.7 > 0.05) at the significance level of 5%. Normally planed (with sharp knives) and coarsely micro-structured produce surfaces significantly different in terms of roughness ( = 1.06 ⋅ 10 −7 < 0.05). The fine microstructuring also showed a significant difference compared to the normal planing ( = 1.37 ⋅ 10 −2 < 0.05).

Tensile Shear Strength
In the dry stage, the normally planed boards yielded the best performance results. However, the measured tensile shear strength relates more to the wood, as the proportion of broken wood was very large. The coarsely micro-structured specimens showed the secondhighest tensile shear strength (around 15 MPa) and the lowest dispersion (see Figure 4). This low dispersion is due to the low wood failure percentage (WFP). For sanding, the dispersion was the highest, although the mean value was above the 15 MPa line, which can be explained by the high dispersion in the wood failure percentage (WFP). When the WFP is close to 100% in a dry test, the measured tensile shear strength corresponds to wood strength. The lowest WFP performance was found in the coarsely micro-structured specimens. Since they had quite high TSS values, it can be concluded that this group performs well in the dry phase. The coarse structure seems to cause a lower wood failure percentage when used with one-component polyurethane adhesive. Both micro-structuring methods and the normal planing were significantly different in terms of the wood failure percentage (Kruskal-Wallis and Dunn's test p = 8.25 × 10 −9 < 0.05 for S1/N and p = 3.62 × 10 −5 < 0.05 for S2/N). The normally planed boards outperformed the other groups in the percentage of wood failure. All samples met the requirements of the dry test.

Tensile Shear Strength
In the dry stage, the normally planed boards yielded the best performance results. However, the measured tensile shear strength relates more to the wood, as the proportion of broken wood was very large. The coarsely micro-structured specimens showed the second-highest tensile shear strength (around 15 MPa) and the lowest dispersion (see Figure  4). This low dispersion is due to the low wood failure percentage (WFP). For sanding, the dispersion was the highest, although the mean value was above the 15 MPa line, which can be explained by the high dispersion in the wood failure percentage (WFP). When the WFP is close to 100% in a dry test, the measured tensile shear strength corresponds to wood strength. The lowest WFP performance was found in the coarsely micro-structured specimens. Since they had quite high TSS values, it can be concluded that this group performs well in the dry phase. The coarse structure seems to cause a lower wood failure percentage when used with one-component polyurethane adhesive. Both micro-structuring methods and the normal planing were significantly different in terms of the wood failure percentage (Kruskal-Wallis and Dunn's test = 8.25 ⋅ 10 −9 < 0.05 for S1/N and = 3.62 ⋅ 10 −5 < 0.05 for S2/N). The normally planed boards outperformed the other groups in the percentage of wood failure. All samples met the requirements of the dry test.  Under wet test conditions, poorly planed specimens are the weakest, showing a much lower average value and a dramatically low median value along with the largest reported dispersion, as shown in Figure 4. The sanded specimens narrowly passed the test. Most of the groups had specimens with a very low WFP. The lowest dispersion in tensile shear strength was observed in coarsely micro-structured specimens. Although all WFP are very close to zero, the adhesion is stable enough to reliably ensure passing the test. The finer structure shows a different behaviour with quite a high dispersion; the second-highest dispersion measured after the dull planed samples. The normally planed surfaces show a slightly better average tensile shear strength value than the sanded one. The dull planed surfaces' tensile shear strength strongly deviates from the normal distribution based on a Shapiro-Wilk normality test (p = 0.04139 < 0.05). A Kruskal-Wallis significance test in combination with a Dunn's post hoc test revealed no significant difference between the groups. The only significant difference was found between the dull planed surfaces and the normally planed surfaces (Dunn's test p = 0.00941 < 0.05) at a significance level of 5%.

Tensile Shear Test Results
Lap joint results for PUR. The left-hand side of Figure 5 shows, from top to bottom sequentially, A1 and A4 test results according to EN 302-1. In the dry stage, the highest bonding strength was obtained for the sharp planed variant with 125 g/m 2 when considering the entire whisker. However, the relatively high dispersion lessens the arithmetical average. In terms of the arithmetical mean of the tensile shear strength, the coarsely microstructured surface with a grammage 200 g/m 2 has the best performance; this variant also shows the lowest dispersion. Most samples have quite a low wood failure percentage. All samples fulfilled the requirements in the dry stage. It is not possible to increase the wood failure percentage of one-component polyurethane by using structural planing. Increasing the adhesive amount slightly improves the WFP values.
In the wet stage, the finely micro-structured surface with a grammage of 125 g/m 2 show the highest arithmetical mean value. Increasing the adhesive amount reduces the bond performance. One group could not reach the tensile shear strength benchmark value defined in EN 15425 (see variant S1 200 g/m 2 ). All groups expect the sharp planed specimens with 125 g/m 2 have WFP values very close to zero.
Statistical investigations showed no significant difference between micro-structuring and normal planing for the grammage of 125 g/m 2 (Welch's ANOVA for A1 p = 0.263 > 0.05 and Kruskal-Wallis p = 0.09001 > 0.05). For the grammage 200 g/m 2 , no significant difference was found at the wet stage (ANOVA test p = 0.475 > 0.05). The dry stage test revealed a significant difference between the coarsely micro-structured and normally planed surfaces (Welch's ANOVA and Games-Howell post hoc test p = 0.013 < 0.05).
Lap joint results for MF. Figure 5 also presents test results of specimens bonded with melamine formaldehyde. In the dry test condition, all samples passed the test since the recorded mean and median values were higher than the minimum required value. The median values were not significantly different regardless of the applied grammage for micro-structured surfaces. It can be observed that increasing the grammage reduces the dispersion within the groups. For all samples, the measured wood failure percentage is high and close to 100%. a reduced adhesive amount, sharp planed surfaces perform better than structural planed surfaces (in wet conditions). Statistical analyses were performed within grammage groups for A1 and A4 treatment. Welch's ANOVA and a Games-Howell post hoc test showed a significant difference between normally planed and finely micro-structured surfaces for a grammage of 250 g/m 2 ( = 0.002 < 0.05). For 400 g/m 2 , there was a significant difference noticed between both micro-structuring methods (for S1/S2 = 0.0285 < 0.05 Kruskal-Wallis and Dunn's post hoc test). For the same grammage, in dry conditions, no significant differences were observed.

Delamination Results
The results of the tested delamination specimens are grouped in Figure 6. No sample bonded with PUR passed the test. Even both reference glulams showed much higher delamination values than the approved delamination.
Delamination results for MF bonded samples are presented in Figure 7. Both microstructured glulams fulfilled the delamination requirement according to EN 302-1 for type I adhesives without closed waiting time. The reference glulam (normally planed) glued with 250 g/m 2 with a closed assembly time of 20 min did not pass the delamination test since its In the wet stage, all groups of specimens delivered satisfying tensile shear strength values. No significant difference between micro-structured surfaces and normally planed surfaces in terms of wood failure percentage was noticed. The smoothest surface bond with 400 g/m 2 with no waiting time (CAT = 0 min) yielded the best bond performance. For a reduced adhesive amount, sharp planed surfaces perform better than structural planed surfaces (in wet conditions).
Statistical analyses were performed within grammage groups for A1 and A4 treatment. Welch's ANOVA and a Games-Howell post hoc test showed a significant difference between normally planed and finely micro-structured surfaces for a grammage of 250 g/m 2 (p = 0.002 < 0.05). For 400 g/m 2 , there was a significant difference noticed between both micro-structuring methods (for S1/S2 p = 0.0285 < 0.05 Kruskal-Wallis and Dunn's post hoc test). For the same grammage, in dry conditions, no significant differences were observed.

Delamination Results
The results of the tested delamination specimens are grouped in Figure 6. No sample bonded with PUR passed the test. Even both reference glulams showed much higher delamination values than the approved delamination. delamination value was slightly higher (5.13%) than the admitted maximal value, whereas the other reference sample with only 400 g/m 2 passed the test.

Tool Life
The frequency with which knives need to be changed is very crucial for the industry. Change and set-up times can significantly affect the overall productivity of the plant. In this project, less than 300 linear metres were planed. Observing wear indicators in such a short operation (low number of planed samples) poses a challenge for industrial implementation (see Figures 8 and 9). The productivity gained by shortening the bonding time can be lost again due to tool-change times. Delamination results for MF bonded samples are presented in Figure 7. Both microstructured glulams fulfilled the delamination requirement according to EN 302-1 for type I adhesives without closed waiting time. The reference glulam (normally planed) glued with 250 g/m 2 with a closed assembly time of 20 min did not pass the delamination test since its delamination value was slightly higher (5.13%) than the admitted maximal value, whereas the other reference sample with only 400 g/m 2 passed the test.
Forests 2022, 13, x FOR PEER REVIEW 12 of 18 delamination value was slightly higher (5.13%) than the admitted maximal value, whereas the other reference sample with only 400 g/m 2 passed the test.

Tool Life
The frequency with which knives need to be changed is very crucial for the industry. Change and set-up times can significantly affect the overall productivity of the plant. In this project, less than 300 linear metres were planed. Observing wear indicators in such a short operation (low number of planed samples) poses a challenge for industrial implementation (see Figures 8 and 9). The productivity gained by shortening the bonding time can be lost again due to tool-change times.

Tool Life
The frequency with which knives need to be changed is very crucial for the industry. Change and set-up times can significantly affect the overall productivity of the plant. In this project, less than 300 linear metres were planed. Observing wear indicators in such a short operation (low number of planed samples) poses a challenge for industrial implementation (see Figures 8 and 9). The productivity gained by shortening the bonding time can be lost again due to tool-change times. 2022, 13, x FOR PEER REVIEW 13 of 18

Roughness
The normally planed surface shows lower roughness than the dull-planed and sanded surfaces. Kläusler et al. [14] carried out similar investigations on beechwood (Fagus sylvatica L.) and came to the same conclusions. They reported that sharp planing gives the smoothest surfaces, followed by fine sanding and dull planing. In their investigations, they used much smoother planing, as the feed f z was 0.5 mm. This contrasts with the feed rate of 1.4 mm selected for the thickness planer used for this project (see Table A1). The four-face-planer had a less-harsh feed ( f z = 1.13 mm) with less-deep planing strokes, which certainly also contributed to smoothing the roughness. Although the coarsely microstructured (S1) series had the roughest surface, it did not give the best results in the tensile shear test. This illustrates once again why it is not obvious to fully predict the bonding quality based on roughness as a surface parameter.
The Ra value of 15 µm with P100 sandpaper seems to be quite high compared to what Kläusler et al. [14] obtained for surfaces sanded with P120. The difference is probably due to different sanding parameters. Hernández and Cool [37] found a different behaviour for a lighter hardwood-birch. They reported that sharp planing had a greater roughness than sanding in three successive stages with grits 100-120-150. The choice of such a fine grit is understandable, as their study aimed to optimise the wood coating.

Tensile Shear Test
Dry stage. All surfacing methods could pass the shear test in dry testing conditions. This result is consistent with what has already been found in previous research projects. It has been reported that even poorly planed boards performed well in this stage [2,14]. The significance of an A1 test (according to EN 302-1 Table 1) is impaired by the high wood failure percentage. The considerable dispersion observable on the poorly planed samples can be explained by the irregularities associated with dull knives that are not evenly damaged.
Wet stage. In wet testing conditions, all groups had a wood failure percentage near zero. This shows that the failure behaviour of the wood with one-component polyurethane (without primer) cannot be reliably influenced by the choice of a particular surface-preparation method. This observation was already made in another study that investigated 1C-PUR [16]. It could also be observed that samples planed with sharp knives deliver better results than the sanded specimens. This result is in agreement with other studies carried out on different types of wood [14,15,21]. Nevertheless, damaged cells could not be observed by fluorescence microscopy, such as in Murmanis et al. [21]. This is due to the fact that they used a very coarse grain size (36) and worked on lightweight deciduous species. For dense hardwood such as beech, it is not easy to observe machining impact using light microscopy. The relatively recent study by Kiliç [15] showed that excessive roughness reduces the shear strength of PUR and PVAc adhesives, with the surface produced with a circular saw giving the lowest result, while the sharply planed surface showed the best performance. This agrees with the observation that the finely micro-structured surfaces have a better bond performance in wet conditions than the coarsely micro-structured specimens since the coarser pattern gives rougher surfaces. Tracking the roughness of surfaces can help understand the behaviour of the adherends.  [2] already reported. There were discrepancies between the relatively low wood failure and the observed strength for some groups. A similar observation was also reported in the literature [38]. Differences in bond strength might also be related to the differences in density between the samples [2]. However, the samples were chosen according to EN 302-1 to reduce this effect.
Wet conditions. Except for one-component polyurethane adhesives without chemical pre-activation, the wood failure percentage was very low. One-component polyurethane is reported to have insufficient water resistance when not treated by a suited priming solution [12,39]. As the adhesive amount increases, the dispersion within the different groups of micro-structured boards decreases. For normally planed surfaces, a different phenomenon is observed. Both the WFP and TSS are significantly lower for higher grammage. This observation is unexpected since both groups are in the same range of density. The observations made in both test results (in dry and wet conditions) show that there is no clear positive influence on bond strength when using structural planing on one-component polyurethane-bonded lap joints. It is also clear that the wood failure percentage of onecomponent polyurethane cannot be influenced by changing the machining method [38]. Structural planing combined with polyurethane cannot impact the wood failure percentage. Furthermore, having micro-structured samples quite close to the minimum accepted resistance value for the wet-stage test indicates that structural planing without a priming solution in combination with a fast-reacting 1C PUR does not significantly improve bond performance.
Melamine formaldehyde. Melamine formaldehyde yielded much higher wood failure percentage values in the dry stage, as expected [2,40]. In studies using MUF wood, a failure percentage higher than 70% was achieved in dry conditions. Such a clear wood failure percentage is an indicator of good bond quality. In dry conditions, for similar WFP values, micro-structured surfaces perform better than normally planed samples; this is in agreement with what was assumed based on the literature [3].
In wet testing conditions, the wood failure percentage was much lower. Most groups had WFP values much lower than the benchmark of 70%. Those observations corroborate the conclusion of Kläusler et al. [5] since they declared that the wood failure percentage could not be improved by simply changing the machining methods employed to generate the surface. For both adhesive systems, the one-component polyurethane and melamine formaldehyde adhesive, the same trend can be observed: for most variants, the finely micro-structured surfaces have slightly better results. This behaviour can be attributed to the positive effect of little roughness, as theorised by Sogutlu [41].

Delamination
Polyurethane. A positive influence of micro-structuring could not be found in these data, contrary to what was found in the literature [3]. This difference is caused by the short open time of the adhesive used during this project. A primer solution cannot be replaced by structural planing. As expected, the normally planed surfaces without primer clearly did not pass the delamination test. Many studies have established the importance of chemical pre-treatment of hardwood [2,12,39,42]. The micro-structured glulams delivered even worse results than the normally planed glulams used as reference. The reason for this behaviour may lie in the difference in roughness [41]. Furthermore, the positive effect of roughness can be an additional explanation. De Moura and Hernández [22] reported better ageing behaviour for surfaces with lower roughness when they compared sanded to planed surfaces. Roughness is limited to the surface, but damage just below the wood surface can also affect the delamination resistance [11]. Subsurface analysis might deliver key information to better grasp the impact of micro-structuring on hardwood.
Melamine formaldehyde. The noticed positive influence of micro-structuring on melamine-formaldehyde-bonded glulams could also be observed in the delamination results since it was possible to pass the test without observing a closed assembly time. This confirms the results of Lehmann and Volkmer [3]. The finer structure also delivered better results, as observed in the shear test in wet conditions. The significant difference observed through statistical testing supports this observation. Mechanisms behind the improvement of bond quality when using micro-structuring cannot only be associated with the increase of the area. Therefore, it was not possible to pass the test with a lesser adhesive amount (grammage significantly lower than the recommended amount). On the contrary, for reduced grammage, micro-structuring effectively decreases the bond resistance. For melamine formaldehyde, micro-structuring can effectively improve the glueing process. Furthermore, the results are consistent with the findings from the tensile shear strength tests in the wet stage, which showed that finely micro-structured surfaces performed better.

Conclusions
The aim of the present research work was to evaluate the effects of structural planing on beechwood (Fagus Sylvatica L.). Based on the results observed during the different activities of this project, the following conclusions can be drawn: Micro-structuring in combination with a small amount of adhesive leads to poor bonding quality in both dry and wet conditions. Structural planing does not effectively increase the percentage of wood failure. In this respect, this machining method is like the reported methods (sanding, planing with sharp knives, planing with dull knives). The adhesive and the wood seem to have a greater influence. Furthermore, micro-structuring does not significantly affect tensile shear strength in the wet stage.
The roughness analysis of the micro-structured surfaces shows that the size of the pattern can significantly influence the measured roughness.
For melamine formaldehyde adhesive, structural planing replaces the observation of the closed waiting time. The mechanisms leading to this behaviour are still unknown, as the micro-structuring was no longer visible on the adhesive joints that successfully passed the delamination test. For example, it is still unclear why the structure is not observable on some adhesive joints with deep delaminating stabilities while it completely merges into the adhesive joint on high-performing bonds. Further microscopic analysis should be carried out to investigate the substrate. The effects of pressure on the textured, planed surfaces should also be investigated.
One-component polyurethane structural planing yielded very high delamination values. This shows that structural planing cannot replace a chemical pre-treatment of the hardwood surface to improve the bonding quality, given the current state of knowledge. Structural planing cannot enable the faster glueing of hardwood when using polyurethanebased adhesive if primer is avoided.
The micro-structured knives used in this study tend to break and wear more quickly than conventional knives. For further research, projects using knives with superior tool service life should be considered.  Data Availability Statement: Data reported in this study can be found in onedrive link to the data supporting the results.