Abstract
Haze control cost is hard to value by a crisp number because it is often affected by various factors such as regional uncertain meteorological conditions and topographical features. Furthermore, regions may be involved in different coalitions for haze control with different levels of effort. In this paper, we propose a PM2.5 cooperative control model with fuzzy cost and crisp coalitions or fuzzy coalitions based on the uncertain cross-border transmission factor. We focus on the Beijing–Tianjin–Hebei regions of China and obtain the following major findings. In the case of haze control in the Beijing–Tianjin–Hebei regions of China, local governments in the global crisp coalition can achieve their emission reduction targets with the lowest aggregated cost. However, Hebei fails to satisfy its individual rationality if there is no cost sharing. Therefore, the Hukuhara–Shapley value is used to allocate the aggregated cost among these regions so that the grand coalition is stable. However, the Beijing–Tianjin–Hebei regions cannot achieve their emission reduction targets in the global fuzzy coalition without government subsidies.
1. Introduction
Air pollution is a global problem. Many countries are suffering from haze, such as Mongolia, Pakistan, Saudi Arabia, Egypt, Iran, and China. Haze control is an urgent and difficult task. “Free riding” can be inevitable in haze control due to the negative externalities of cross-border transmission between regions. So, how to balance the interests of multiple parties with an effective cost-sharing mechanism is a key issue. However, it is hard to model air pollution with crisp values because there are all kinds of uncertain information. The transmission rate is difficult to estimate accurately. For example, 28–36% PM2.5 of Beijing was transmitted from non-Beijing area [1]. Hence, the direct cost of haze control and the impact of haze control on a region’s economic development cannot be accurately determined. Furthermore, the information among players can be asymmetric and vague in a cooperative game because the players, in order to achieve a favorable outcome, may conceal key information such as their pollution discharge and management. Moreover, the players also may be involved in different coalitions with different levels of effort at the same time because of their limited economic resources [2]. This may result in fuzzy coalitions with incomplete participation among the players.
Zadeh [3] proposed a fuzzy set is a class of objects with a continuum of grades of membership. And the notions of inclusion, union, intersection, complement, relation, convexity, etc., are extended to such sets. Since then, there have been a great number of applications of fuzzy sets. In the literature on the prediction, monitoring, and control of air pollution, Guo et al. [4] and Shad et al. [5] used fuzzy spatial prediction techniques to determine pollution concentration areas in practical situations where observations are imprecise and vague that improved the prediction accuracy and real-time of the air pollutant concentration prediction. Wang et al. [6] developed a novel early warning system based on fuzzy time series to forecast the major air pollutants considering the large fluctuations in the concentration of pollutants. Souza [7] studied the automation of air pollution monitoring using genetic algorithm, fuzzy logic, and neural networks for data from nuclear techniques analysis of industrial waste. Li et al. [8] built a dynamic evaluation model for the purpose of mastering the future air quality immediately based on the method of fuzzy mathematical synthetic evaluation. Fisher [9] illustrated ways in which concepts from fuzzy set theory may be applied to decision-making in the environmental sciences. Later, Zhen et al. [10] and Chen et al. [11] proposed interval-parameter fuzzy programming mixed integer programming method and energy-environment optimization model based on fuzzy set theory, which provided solutions for more efficient pollution reduction. Centobelli et al. [12] proposed the adoption of fuzzy set theory in the field of supply chain and designed a fuzzy-based decision support system. Fan et al. [13] proposed a Stackelberg game model to investigate the profit changes of two coal-electricity price linkage (CEPL) mechanisms caused by different production strategies of coal mining enterprises and coal-fired power plants when coal prices rise to mitigate the serious conflicts between market-driven coal prices and state-administered electricity prices. Some scholars combine fuzzy set theory with game theory to study public goods, such as water resources management. Armaghan [14] studied the optimal allocation of water resources across river basins from the perspective of fuzzy cooperative games. Two fuzzy cooperative game models were established based on water users’ uncertainty of fuzzy income functions and their fuzzy participation degree of coalitions. The results showed that the global coalition resulted in the highest benefit. Armahan [15] further considered political factors to the net income redistribution of the coalition that indicate that considering political factors can provide a solution that makes all water users more satisfied. Moreover, existing studies [16,17,18] provided valuable suggestions for solving water conflicts by using fuzzy cooperative game theory to the water allocation of China’s South-to-North Water Transfer Project. Water resources and haze are both public goods with externality and non-excludability. Hence, the fuzzy cooperative game model is also applicable to haze control. However, a major difference is that water flow is one-way cross-border transmission while haze transmission is bi-directional. So far, limited studies have applied fuzzy game into haze control. Zhou et al. [19] introduced haze cost with interval number and allocated aggregated cost of global coalition by the interval Shapley value. The coalition is vague while the control cost is certain. Sun [20] established a cooperative game model with fuzzy participation and designed an economic benefit coordination mechanism for haze control. However, research is lacking on air pollution with fuzzy cost and fuzzy coalition. The existing studies on PM2.5 emission reduction strategies are based on regional total control principle. This means as long as the total amount of regional pollution is up to an abatement request, it is assumed that all regions meet the standards. Such an assumption can lead to “free riding” by some regions, making the emission reduction inefficient. Therefore, the conclusions, and hence the proposed policies from the existing studies, may be unreliable.
There are three contributions in this paper. First, we model the impact of PM2.5 emissions with fuzzy cost and fuzzy coalition. Second, we adopt the concentration control principle and consider the impact of regional transmission factors. Third, we provide practical managerial and policy implications for haze control in China and other countries.
The structure of the paper is as follows. In Section 2, the fuzzy aggregated cost function of PM2.5 control is constructed. Section 3 establishes a cooperative game model with fuzzy cost and crisp coalition and a cooperative game model with fuzzy cost and fuzzy coalition. Section 4 conducts a case study of the Beijing–Tianjin–Hebei regions in China. Conclusions and policy insights for intergovernmental cooperation on PM2.5 as well as future research directions are presented in Section 5.
2. Preliminary Conceptions
2.1. Preliminary of Interval Numbers
Definition 1.
If , it is called a standard binary interval number, or interval number in short, where, and represent the lower and upper limits of the interval number, respectively.
Definition 2.
Assume and are fuzzy numbers. If there is a fuzzy number such that , then the Hukuhara-difference of and exists. is called Hukuhara-difference, which is simply the H-difference, recorded as .
Operation 1.
For any interval numbers , , , there are the following rules of operation:
The basic operation of the interval number is a closed operation.
2.2. Symbols
Symbols and descriptions of the paper are in Table 1.
Table 1.
Symbols and description.
Assuming regions, the fuzzy reduction of PM2.5 in region is:
where and are the production and removal of PM2.5 in the region, respectively. and are the production and removal of last year in the region , respectively. is the fuzzy contribution rate to region by the PM2.5 emission of region . indicates its own local influence. The fuzzy contribution rate of PM2.5 from region to region is calculated as follows:
where represents the fuzzy interval transmission ratio of the average annual PM2.5 concentration of region to region . is the conversion coefficient between the mass and the concentration of the region PM2.5. is the annual average concentration of PM2.5 of the region . If there is a conversion relationship between the removal and the concentration of PM2.5, and the conversion coefficient is , then the relationship between the fuzzy reduction amount of PM2.5 and the fuzzy falling concentration is:
3. PM2.5 Cooperative Control Model with Fuzzy Cost and Fuzzy Coalitions
3.1. The Uncertain Aggregated Cost Function of PM2.5 Control
Since the source of PM2.5 is mainly affected by gaseous precursors of SO42− and NO3− [21], the control of SO2 and NOX instead of PM2.5 are studied in the paper. The emission reductions of SO2 and NOX are all denoted by the interval numbers due to the fuzzy cross-border transmission rate of PM2.5. According to Tan et al. [22], the fuzzy control cost function of SO2 is:
where is the fuzzy control cost of SO2 in the region , is the exhaust emission of the region , is the fuzzy removal of SO2 in the region , and are the parameters to be determined. According to [23], the fuzzy control cost function of NOX can be constructed as follows:
where is the fuzzy control cost of NOX in region , is the unit fuzzy control cost, and is the fuzzy removal amount of NOX in region . Therefore, the direct control cost function of PM2.5 with uncertain information for region is:
where is the fuzzy direct control cost of PM2.5 for region . and are the conversion coefficients between SO2 and NOX removal and concentration for region , respectively. Haze control also may have a certain degree of negative impact on economic development in the control process. Li et al. [24] derived the impact of environmental regulation on 41 industries from the CGE model. The aggregated cost of environmental regulation is:
where is the impact of environmental regulation on industry S, and is the annual output value of industry S in region . The fuzzy economic development impact function of region is:
where represents the economic loss caused by the unit concentration of PM2.5 per year in region , and is the time factor. The uncertainty of aggregated control cost is the sum of fuzzy direct control cost and economic development impact cost, so the regional uncertain aggregated cost function is:
3.2. Fuzzy Cooperative Game Model with Crisp Coalition
According to Borkotokey [25], there are many types of uncertainties when forming coalitions. In many cases, players can only make vague judgments about the true value of the coalition. Here players are local governments. Coalition means the group negotiating to strive together to reduce emissions. In a crisp coalition, players participate in a coalition with 100% degree of participation, but in a fuzzy coalition, the degree of participation that means players join in a coalition is between 0% and 100%. The central government has set emission reduction concentrations for each region called Emission Reduction Target (ERT). If each player in the coalition can reach its own ERT within the capability of emission reduction, (10) is held. If not, the players must pay control costs to nearby regions in order to achieve the ERT by cutting down the cross-border transmission emission.
Considering the information uncertainty in the coalition, a fuzzy characteristic function denoted by represents the value of a coalition. Moreover, the regional emission reduction cannot exceed the emission reduction cap. Therefore, the fuzzy characteristic function of a coalition can be represented as:
In the crisp coalition with transferable payment, set represents the global coalitions of all regions participating in the PM2.5 cooperative control. represents the set of all non-empty subsets of the participant set N, i.e., the set of all alliances. S is a subset of N, i.e., . represents the aggregated cost of coalition S and . The Hukuhara–Shapley function [26] is defined as:
where is the number of players in the coalition S and is the benefit distribution value of the coalition players. is the added benefit for the coalition after joining the coalition S. The cost sharing satisfies the individual rationality as well as the collective rationality .
3.3. Fuzzy Cooperative Game Model with Fuzzy Coalition
In a fuzzy coalition, players may participate in a coalition with less than a 100% degree of participation. In the payment-transferable fuzzy Coalition , denotes a subset of all fuzzy coalitions, and fuzzy Coalition , . Let be the participation of in the fuzzy coalition , ; is denoted as the number of elements in the set ; that is, the elements in . is arranged in increasing order, i.e., . Sun and Zhang [27] defined the characteristic function of a fuzzy cooperative game with uncertain Choquet integral form as:
The basic form of the Hukuhara–Shapley function is defined as (13) in Section 3.3. For the fuzzy Coalition, the Hukuhara–Shapley function with the uncertain Choquet integral form [26] is defined as:
where is the cost of player joining the fuzzy coalition with participation .
4. Case Study
4.1. Overview of the Beijing–Tianjin–Hebei Regions Air Pollution
Since 2013, haze has frequently occurred in North China, especially in the Beijing–Tianjin–Hebei regions. Air pollution has attracted the attention of the central government and scholars. Fan et al. [28] analyzed several drivers of carbon dioxide emissions using the decomposition analysis method based on input and output(IO-SDA) and provided policy advice for low carbonization in the Beijing-Tianjin-Hebei regions. And the Beijing Environmental Protection Monitoring Center has monitored PM2.5 concentration from 2013. The central government has set ERTs for Beijing, Tianjin, and Hebei. According to central government request, the goal of Beijing’s 2018 action plan is to continue to strive for a decline in annual average PM2.5, and to set this goal also for each district. The average concentration reduction in Beijing in 2018 is about 1 μg/m3. In addition, the concentrations abatement of Tianjin and Hebei are 1 μg/m3 and 4 μg/m3, respectively.
As the central government’s ERT is the concentration abatement, it is necessary to convert the decrease of concentration into removal amount. According to the study of the atmospheric environmental capacity of various pollutants by Xue et al. [29], the concentration of PM2.5 that can be accommodated in the environmental capacity of 104 tons in the regions of Beijing, Tianjin, and Hebei should be obtained. That is, the conversion coefficients between the removal and concentration of PM2.5 in the Beijing, Tianjin, and Hebei regions are , , and , respectively (for convenience, we use subscript 1, 2, and 3 to represent Beijing, Tianjin, and Hebei, respectively).
The PM2.5 fuzzy transmission matrix shown in Table 2 is calculated using (4) and the PM2.5 space transportation matrix published by the Ministry of Environmental Protection of China includes data from China’s 31 provinces and regions including Beijing, Tianjin, Hebei, Shanxi, and Shandong. The detailed calculation is shown in Table A1, Table A2, Table A3 and Table A4 of Appendix A.
Table 2.
PM2.5 emission transfer matrix of the Beijing–Tianjin–Hebei regions to other regions (%).
In this paper, the logarithmic regression model predicts the amount and removal mass of PM2.5 in 2015. The detailed calculation is shown in Table A5 and Table A6 of Appendix A. According to Xue et al. [30], the upper limit of PM2.5 removal is 95% of PM2.5 production. Therefore, the upper limit of PM2.5 removal in Beijing, Tianjin, and Hebei should be 15.65 tons, 15.78 tons, and 93.68 tons, respectively. Moreover, the basic PM2.5 removal (PM2.5 emission reductions in 2015) are 13.34 tons, 11.37 tons, and 62.45 tons, respectively.
4.2. PM2.5 Uncertain Aggregated Control Cost Function
The industrial waste gas emissions, the industrial SO2 removal in the Beijing–Tianjin–Hebei regions and the control cost of industrial SO2 from 2003 to 2010 in China were selected for calculation. According to (4), the control costs of SO2 in three regions can be obtained. The functions for Beijing, Tianjin, and Hebei are , , and , respectively.
The power industry is the largest source of NOX emission. Liu [31] found that the control cost of a power plant using Selective Catalytic Reduction (SCR) technology NOX is about 1.40–1.61 $/kg. Based on the uncertainty of NOX control cost, the NOX fuzzy control cost functions of the three regions are:
Therefore, the fuzzy direct control cost functions of the three regions of Beijing–Tianjin–Hebei can be obtained from Equation (6):
According to the output value of various industries of the Beijing–Tianjin–Hebei regions in 2015, the aggregated cost of environmental control can be obtained. From Equation (7), the economic loss caused by reducing 104 tons of PM2.5 in each region can be obtained (the time factor is set to the GDP growth rate of each region). Therefore, the influence functions of the Beijing–Tianjin–Hebei regional fuzzy economic development are:
According to Equation (9), the cost functions of PM2.5 uncertain aggregated control in Beijing–Tianjin–Hebei regions are:
4.3. Results and Analysis
When forming a crisp coalition, the three regions of Beijing, Tianjin, and Hebei join the coalition with 100% participation. The crisp coalitions in this paper have the following forms: Individual control, partial coalitions, and global coalition. The fuzzy characteristic functions of the crisp coalitions are represented by the number of intervals.
When Beijing controls PM2.5 individually, Beijing’s emission reduction is = [13.41, 13.38] tons which is less than its emission reduction capacity cap of = 15.64 tons. According to Equation (10), Beijing can complete its target by controlling PM2.5 individually. The fuzzy characteristic value of Beijing is [11.66, 12.73] billion dollars based on Equation (11). Similarly, according to Equation (11), the value of Tianjin and Hebei can be calculated as = [23.95, 25.46] billion dollars and = [65.66, 75.99] billion dollars, respectively.
When Beijing and Tianjin cooperate, Beijing’s emission reduction is = [13.29, 15.64] tons and Tianjin’s emission reduction is = [11.88, 13.68] tons. According to Equation (10), they both can achieve ERTs within their emission reduction capacity. Beijing and Tianjin’s emission reduction capacity caps are = 15.64 tons and = 15.78 tons, respectively. The fuzzy characteristic value of partial cooperation between Beijing and Tianjin is [38.64, 42.32] billion dollars, and the fuzzy cost of individual control in Hebei is [65.66, 75.99] billion dollars.
When Beijing and Hebei cooperate, both can reach the ERTs. The fuzzy characteristic values of partial cooperation between Beijing and Hebei are [77.04, 88.36] billion dollars, and the cost of Tianjin’s individual control is [23.95, 25.46] billion dollars. When Tianjin and Hebei cooperate, they can reach the ERTs as well. The fuzzy characteristic value of Tianjin and Hebei partial cooperation is [89.03, 99.79] billion dollars, and Beijing’s control cost is: [11.66, 12.73] billion dollars.
When the Beijing–Tianjin–Hebei regions reach a global coalition, the emission reduction in the three regions is = [12.70, 13.10] tons, = [10.79, 11.31] tons, and = [71.20, 77.70] tons. According to Equation (10), it can be concluded that all three regions can achieve ERTs within their emission reduction capacity. The fuzzy characteristic value of the global coalition is [100.42, 112.19] billion dollars, of which Beijing’s control cost is [11.37, 11.95] billion dollars, Tianjin’s control cost is [23.27, 23.35] billion dollars, and Hebei’s control cost is [65.70, 76.98] billion dollars.
By calculating the fuzzy characteristic value of various coalitions based on Equation (11), these coalitions’ aggregated costs can be obtained. To determine which coalition is the best based on the principle of cost minimization, the sum of the aggregated costs of Beijing–Tianjin–Hebei regions in each coalition form is computed as Table 3. It can be concluded that the aggregated cost of the Beijing–Tianjin–Hebei regions is the smallest with global coalition cooperation. Hence, the global coalition is the best control method. For the members of the coalition, the control costs of Beijing and Tianjin have declined through cooperative control, but the cost of control in Hebei is higher than that of individual control. Therefore, it is necessary to distribute the control costs fairly to achieve a stable global coalition in the long term. The fuzzy eigenvalue table of the cooperative game of the crisp coalition is summarized as below in Table 4.
Table 3.
The sums of the aggregated costs in various coalition forms (billion dollars).
Table 4.
Fuzzy eigenvalue table of the cooperative game of crisp coalition (billion dollars).
The Hukuhara–Shapley value is used to share the aggregated cost of global cooperative control. According to Equation (12), Beijing’s cost allocation by joining the global coalition is:
Similarly, Tianjin’s cost allocation in the global coalition is [24.24, 25.33] billion dollars. Hebei’s cost allocation in the global coalition is [64.18, 73.61] billion dollars.
The results associated with the fuzzy cooperative game model with crisp coalition are summarized in Table 5. It can be seen that after the Hukuhara–Shapley value distribution, Hebei’s control cost is less than the cost of individual control, so joining the global coalition satisfies its individual rationality. Similarly, joining the global coalition is also the best choice for Tianjin. Geographically, Beijing is only connected to Hebei and Tianjin, so Beijing’s non-local emissions are mainly from Hebei and Tianjin. Although Beijing’s control cost of joining the global coalition is slightly higher than its individual control. However, global cooperation control effectively avoids repeated pollution of haze, and helps with emission reduction in Beijing. Thus, Beijing is willing to join the global coalition. Therefore, the global coalition is the best. The aggregated cost of the global coalition is [100.42, 112.19] billion dollars. The control costs in Beijing, Tianjin, and Hebei are [11.98, 13.25] billion dollars, [24.24, 25.33] billion dollars, and [64.18, 73.61] billion dollars, respectively.
Table 5.
Comparison of the aggregated costs in individual and global coalition (billion dollars).
The developed regions usually pay more attention to environmental protection. Therefore, economic development level is a key factor in haze control. Considering the actual economic development level, Beijing joined the coalition with 100% participation, while Tianjin and Hebei could not fully join the coalition. That is, they joined the coalition with a certain degree of participation. Next, the fuzzy cooperative game model with fuzzy coalition will be discussed. We assume the participation results of the Beijing–Tianjin–Hebei regions are presented in Table 6.
Table 6.
Participation degree of cooperation control in the Beijing–Tianjin–Hebei regions.
According to the characteristic function of fuzzy cooperative game with uncertain Choquet integral form as in (13), the fuzzy characteristic functions of fuzzy coalition are calculated, which are presented in Table 7.
Table 7.
Fuzzy eigenvalue table of cooperative game of fuzzy coalition (billion dollars).
Under the fuzzy coalition, the following results are derived based on Equation (12):
Similarly, [17.25, 18.17] billion dollars and [32.09, 36.81] billion dollars. According to Equation (14), Beijing’s cost allocation in the global fuzzy coalition is:
Similarly, the cost allocations of Tianjin and Hebei to the global fuzzy coalition are [15.26, 16.37] billion dollars and [34.11, 39.10] billion dollars, respectively.
The above results show that Hebei has the highest cost of control in the fuzzy coalition, followed by Tianjin, and then Beijing. In the case of fuzzy coalition, with the participation degree of 100%, Beijing needs to bear the control cost of [6.05, 6.70] billion dollars. Tianjin’s control cost under the participation degree of 0.7 is [15.26, 16.37] billion dollars. And Hebei’s control cost under the participation of 0.5 is [34.11, 39.10] billion dollars. Moreover, the minimum control costs of the three regions, Beijing, Tianjin, and Hebei, are [11.98, 13.25] billion dollars, [24.24, 25.33] billion dollars, and [64.18, 73.61] billion dollars, respectively, when each player’s participation is 1 and the central government’s ERTs are met. Comparing to the control costs under the crisp coalition and the fuzzy coalition, none of the players can meet the ERTs set by the central government under the fuzzy coalition. Hence, the central government should support, by providing financial subsidies, for example, local governments to increase the participation degree of haze control.
5. Conclusions
In general, it is a challenging task to evaluate haze control cost of a region using a crisp number. This is because of a variety of information uncertainties and the possible forming of coalitions by regions. Therefore, in this paper, we established a model of PM2.5 cooperative control with fuzzy costs and crisp coalitions or fuzzy coalitions. We then applied our model to the haze control of the Beijing–Tianjin–Hebei regions in China.
Specifically, with the central government’s emission reduction targets (ERTs), it was assumed that each region joins the coalition with 100% participation. The central government established a PM2.5 control cooperation game model with crisp coalition and fuzzy cost, seeking to minimize the costs of local governments and meets ERTs. By calculating the control costs of the global coalition and the partial coalitions, our results show that the global coalition minimizes the aggregated cost. This satisfies the collective rationalities of local governments participating in the global coalition. However, in this case, the control cost of Hebei fails to satisfy its individual rationality. Therefore, in the paper, the Hukuhara–Shapley value was adopted to allocate the aggregated cost of the global coalition according to the marginal contribution, so that each player is willing to join the global coalition. If the local governments are unable to complete the central government’s ERTs within their emission reduction capability caps, the central government can provide subsidies to increase the participation of local governments. Furthermore, as the cross-regional transmission factor changes over time, local government air pollution control expenditures and central government subsidies should also be adjusted accordingly.
There are more than one future research directions for this paper. First, this paper focuses on PM2.5 control in the Beijing–Tianjin–Hebei regions. Further research could consider the interactions among more regions. In such a scenario, a player can join more than one coalition. Second, future research could apply our proposed model to other settings such as water allocation.
Author Contributions
Conceptualization, Z.Z. and M.Z.; methodology, Z.Z. and X.Y.; software, K.W. and J.W.; validation, M.Z.; formal analysis, H.S.; resources, Q.S. and M.Z.; writing—original draft preparation, M.Z. and J.W.; writing—review and editing, Z.Z. and X.H.; visualization, M.Z.; supervision, Z.Z.; funding acquisition, Z.Z., X.Y., and H.S.
Funding
The research is supported by the National Natural Science Foundation of China (NSFC) under the Grant 71874112, 71532002, 71801016, 71871002, and 71771025, Funding by Key Project of the National Social Science Fund: A Study of a New Holistic Governance Framework of Xiongan New Area for the Beijing – Tianjin – Hebei Integrated Development. Approval number 18VSJ066. the Beijing Education Commission Social Science Program general program, the Beijing Natural Science Foundation 4194072 and the Capacity Building for Sci-Tech Innovation—Fundamental Scientific Research Funds of Capital Normal University. The authors would like to thank the valuable reviews and appreciate the constructive suggestions from the anonymous referees.
Conflicts of Interest
The authors declare no conflict of interest.
Appendix A
Calculation of relevant parameters in the cost function:
Appendix A.1. PM2.5 Fuzzy Transmission Rate in the Beijing–Tianjin–Hebei Regions
By reviewing the environmental bulletins of the Beijing–Tianjin–Hebei regions over the years, the annual PM2.5 concentration is constantly changing. According to the source analysis table of PM2.5, the local sources and regional transmission ratios are uncertain. Therefore, PM2.5 space transportation of 31 provinces (autonomous regions and municipalities) announced by the Environmental Planning Institute of the Ministry of Environmental Protection in 2010 and 2015 are applied to represent the PM2.5 fuzzy transmission rate. The regional transmission matrixes extracted from Beijing, Tianjin, and Hebei are as follows:
Table A1.
Local PM2.5 source ratio matrix in the Beijing–Tianjin–Hebei regions in 2010 (%).
Table A1.
Local PM2.5 source ratio matrix in the Beijing–Tianjin–Hebei regions in 2010 (%).
| Sources | Beijing | Tianjin | Hebei | Other Provinces | |
|---|---|---|---|---|---|
| Provinces | |||||
| Beijing | 63 | 4 | 24 | 9 | |
| Tianjin | 6 | 58 | 26 | 10 | |
| Hebei | 5 | 6 | 64 | 21 | |
Table A2.
Local PM2.5 source ratio matrix in the Beijing–Tianjin–Hebei regions in 2015 (%).
Table A2.
Local PM2.5 source ratio matrix in the Beijing–Tianjin–Hebei regions in 2015 (%).
| Sources | Beijing | Tianjin | Hebei | Other Provinces | |
|---|---|---|---|---|---|
| Provinces | |||||
| Beijing | 66 | 4 | 18 | 12 | |
| Tianjin | 3 | 56 | 20 | 21 | |
| Hebei | 3 | 4 | 62 | 31 | |
Based on the uncertain transmission ratio of PM2.5 in the Beijing–Tianjin–Hebei regions, the contribution transmission rate is assumed to be an interval number. The lower limit of the interval is the smaller of the transmission rates of PM2.5 in 2010 and 2015, and the upper limit is the larger of the transmission rates of PM2.5 in 2010 and 2015, the new PM2.5 fuzzy transmission matrix in the Beijing–Tianjin–Hebei regions is obtained:
Table A3.
Local PM2.5 source fuzzy proportional matrix in the Beijing–Tianjin–Hebei regions (%).
Table A3.
Local PM2.5 source fuzzy proportional matrix in the Beijing–Tianjin–Hebei regions (%).
| Sources | Beijing | Tianjin | Hebei | Other Provinces | |
|---|---|---|---|---|---|
| Provinces | |||||
| Beijing | [63,66] | [4,4] | [18,24] | [9,12] | |
| Tianjin | [3,6] | [56,58] | [20,26] | [10,21] | |
| Hebei | [3,5] | [4,6] | [62,64] | [21,31] | |
According to the data released by the Environmental Protection Agency in 2016, the annual average concentrations of PM2.5 in Beijing, Tianjin, and Hebei are 73 μg/m3, 68 μg/m3, and 70 μg/m3 respectively.
According to Equation (2), it can be concluded that the PM2.5 interval contribution matrix of PM2.5 in Beijing, Tianjin, Hebei, and other regions is as follows:
Table A4.
PM2.5 fuzzy emission transfer matrix of the Beijing–Tianjin–Hebei regions and other regions (%).
Table A4.
PM2.5 fuzzy emission transfer matrix of the Beijing–Tianjin–Hebei regions and other regions (%).
| Other Provinces | ||||
|---|---|---|---|---|
| [49.55,55.61] | [2.79,5.21] | [20.22,31.46] | [13.78,21.37] | |
| [2.67,3.07] | [42.27,47.48] | [24.59,31.69] | [23.40,24.86] | |
| [1.86,2.41] | [2.28,2.88] | [31.40,51.32] | [43.31,44.53] |
Appendix A.2. Determination of PM2.5 Removal
In the Beijing–Tianjin–Hebei regions, controlling the emission of SO2 is the key issue of restricting PM2.5, so the amount of PM2.5 can be estimated by the production of SO2. However, the removal of SO2 is no longer provided in the statistical yearbook since 2010, the regression model was used to analyze and predict the removal rate of SO2 from 2003 to 2010, comparing the logarithmic regression model, linear regression model and polynomial regression model, data showed that the logistic regression model had the best regression effect. The logarithmic regression model predicted that the SO2 removal rates of Beijing–Tianjin–Hebei in 2015 were 79.85%, 68.43%, and 63.24%, respectively.
According to the study of the environmental capacity of PM2.5, SO2, and NOX by Xue et al. [19], the corresponding relationship between them is obtained:
Table A5.
Removal of SO2 and NOX corresponding to removal of PM2.5 (×104 tons).
Table A5.
Removal of SO2 and NOX corresponding to removal of PM2.5 (×104 tons).
| Corresponding Pollutant Removal | SO2 | NOX |
|---|---|---|
| Beijing | 2.15 | 3.55 |
| Tianjin | 3.54 | 4.37 |
| Hebei | 3.05 | 3.22 |
From the correspondence in the removal of PM2.5, SO2 and the production of SO2 in 2015, the Beijing–Tianjin–Hebei regions predicted by the log-regression model, the removal of PM2.5 can be derived as follows:
Table A6.
Removal of PM2.5 for the Beijing–Tianjin–Hebei regions in 2015 (×104 tons).
Table A6.
Removal of PM2.5 for the Beijing–Tianjin–Hebei regions in 2015 (×104 tons).
| Regions | PM2.5 Removal | PM2.5 Production |
|---|---|---|
| Beijing | 13.1444 | 16.4597 |
| Tianjin | 11.3683 | 16.6130 |
| Hebei | 62.4445 | 98.7375 |
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