Table of Contents
Molecules, Volume 25, Issue 8 (April-2 2020) – 244 articles
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Cover Story (view full-size image) The research of noble metals containing polyoxometalates is a challenging field that combines smart [...] Read more. The research of noble metals containing polyoxometalates is a challenging field that combines smart synthetic approaches and nontrivial reactivity with wide perspectives for different catalytic applications. The unique combination of ruthenium and polyoxoanions creates a new generation of water oxidation and organic substrates activation catalysts. In this report, we summarized our studies of Ru-atom reactivity inside the POM backbone towards azide. Two reaction pathways result in i) azide-acetonitrile click reaction and ii) azide decomposition. The first pathway produces coordinated tetrazole and the second generates a novel POM complex with a coordinated N2 molecule. Such reactivity is important for the transformation of organic substrates and N2 activation. View this paper.