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Materials 2012, 5(11), 2015-2054; doi:10.3390/ma5112015
Review

Materials-Related Aspects of Thermochemical Water and Carbon Dioxide Splitting: A Review

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Received: 3 September 2012; in revised form: 12 October 2012 / Accepted: 17 October 2012 / Published: 24 October 2012
(This article belongs to the Special Issue Advanced Materials for Water-Splitting)
Download PDF [709 KB, uploaded 24 October 2012]
Abstract: Thermochemical multistep water- and CO2-splitting processes are promising options to face future energy problems. Particularly, the possible incorporation of solar power makes these processes sustainable and environmentally attractive since only water, CO2 and solar power are used; the concentrated solar energy is converted into storable and transportable fuels. One of the major barriers to technological success is the identification of suitable active materials like catalysts and redox materials exhibiting satisfactory durability, reactivity and efficiencies. Moreover, materials play an important role in the construction of key components and for the implementation in commercial solar plants. The most promising thermochemical water- and CO2-splitting processes are being described and discussed with respect to further development and future potential. The main materials-related challenges of those processes are being analyzed. Technical approaches and development progress in terms of solving them are addressed and assessed in this review.
Keywords: water splitting; CO2- splitting; thermochemical cycle; redox material; sulfur cycle; solar power; CO; solar fuels; hydrogen water splitting; CO2- splitting; thermochemical cycle; redox material; sulfur cycle; solar power; CO; solar fuels; hydrogen
This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

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MDPI and ACS Style

Roeb, M.; Neises, M.; Monnerie, N.; Call, F.; Simon, H.; Sattler, C.; Schmücker, M.; Pitz-Paal, R. Materials-Related Aspects of Thermochemical Water and Carbon Dioxide Splitting: A Review. Materials 2012, 5, 2015-2054.

AMA Style

Roeb M, Neises M, Monnerie N, Call F, Simon H, Sattler C, Schmücker M, Pitz-Paal R. Materials-Related Aspects of Thermochemical Water and Carbon Dioxide Splitting: A Review. Materials. 2012; 5(11):2015-2054.

Chicago/Turabian Style

Roeb, Martin; Neises, Martina; Monnerie, Nathalie; Call, Friedemann; Simon, Heike; Sattler, Christian; Schmücker, Martin; Pitz-Paal, Robert. 2012. "Materials-Related Aspects of Thermochemical Water and Carbon Dioxide Splitting: A Review." Materials 5, no. 11: 2015-2054.


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