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Int. J. Mol. Sci. 2011, 12(9), 6357-6366; doi:10.3390/ijms12096357
Article

Recognition-Mediated Assembly of Quantum Dot Polymer Conjugates with Controlled Morphology

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1 Department of Chemistry, University of Massachusetts Amherst, 710 North Pleasant Street, Amherst, MA 01003, USA 2 Department of Chemistry, Middle East Technical University, Ankara 06531, Turkey 3 Department of Physics, University of Massachusetts Amherst, 710 North Pleasant Street, Amherst, MA 01003, USA 4 Glasgow Centre of Physical Organic Chemistry, WestCHEM, School of Chemistry, University of Glasgow, Joseph Black Building, Glasgow G12 8QQ, UK
* Author to whom correspondence should be addressed.
Received: 28 August 2011 / Revised: 20 September 2011 / Accepted: 20 September 2011 / Published: 23 September 2011
(This article belongs to the Special Issue Molecular Self-Assembly 2011)
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Abstract

We have demonstrated a polymer mediated “bricks and mortar” method for the self-assembly of quantum dots (QDs). This strategy allows QDs to self-assemble into structured aggregates using complementary three-point hydrogen bonding. The resulting nanocomposites have distinct morphologies and inter-particle distances based on the ratio between QDs and polymer. Time resolved photoluminescence measurements showed that the optical properties of the QDs were retained after self-assembly.
Keywords: molecular recognition; nanoparticles; hydrogen bonding; self-assembly; nanocomposites; quantum dots molecular recognition; nanoparticles; hydrogen bonding; self-assembly; nanocomposites; quantum dots
This is an open access article distributed under the Creative Commons Attribution License (CC BY 3.0).
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Nandwana, V.; Subramani, C.; Eymur, S.; Yeh, Y.-C.; Tonga, G.Y.; Tonga, M.; Jeong, Y.; Yang, B.; Barnes, M.D.; Cooke, G.; Rotello, V.M. Recognition-Mediated Assembly of Quantum Dot Polymer Conjugates with Controlled Morphology. Int. J. Mol. Sci. 2011, 12, 6357-6366.

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