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Molecules 2017, 22(12), 2127; doi:10.3390/molecules22122127

The Molecular Design of Active Sites in Nanoporous Materials for Sustainable Catalysis

Department of Chemistry, University of Southampton, Highfield Campus, University Road, Southampton SO17 1BJ, UK
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Author to whom correspondence should be addressed.
Received: 2 November 2017 / Revised: 23 November 2017 / Accepted: 28 November 2017 / Published: 2 December 2017
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Abstract

At the forefront of global development, the chemical industry is being confronted by a growing demand for products and services, but also the need to provide these in a manner that is sustainable in the long-term. In facing this challenge, the industry is being revolutionised by advances in catalysis that allow chemical transformations to be performed in a more efficient and economical manner. To this end, molecular design, facilitated by detailed theoretical and empirical studies, has played a pivotal role in creating highly-active and selective heterogeneous catalysts. In this review, the industrially-relevant Beckmann rearrangement is presented as an exemplar of how judicious characterisation and ab initio experiments can be used to understand and optimise nanoporous materials for sustainable catalysis. View Full-Text
Keywords: Beckmann rearrangement; characterisation; structure-property correlations; zeotypes; acid sites Beckmann rearrangement; characterisation; structure-property correlations; zeotypes; acid sites
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This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. (CC BY 4.0).

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Chapman, S.; Potter, M.E.; Raja, R. The Molecular Design of Active Sites in Nanoporous Materials for Sustainable Catalysis. Molecules 2017, 22, 2127.

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